The DOI matches its Crossref record; 14 of the 14 references it cites were found in a registry or an index.
Charge-Redistribution-Enhanced Nanocrystalline Ru@IrOx Electrocatalysts for Oxygen Evolution in Acidic Media
Open accessAbstract
Summary Achieving high activity and long-term stability is a major challenge in the design of catalysts. In particular, the oxygen evolution reaction (OER) in acidic media, which plays a key role in proton exchange membrane electrolyzers for fast hydrogen fuel generation, seriously suffers from rapid degradation of catalysts as a result of the harsh acidic and oxidative conditions. Here, we report a rational design strategy for the fabrication of a heterostructured OER electrocatalyst (Ru@IrOx) that has unique physicochemical properties and in which a strong charge redistribution exists between a highly strained ruthenium core and a partially oxidized iridium shell across the metal-metal oxide heterojunction. The increased valence of the iridium shell and the decreased valence of the ruthenium core activate a synergistic electronic and structural interaction, which results in the enhanced activity and stability of the catalyst compared with the majority of the state-of-the-art ruthenium- and iridium-based materials.
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Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
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Cited by
Chen, F.-Y., Wu, Z.-Y., Adler, Z., & Wang, H. (2021) · Joule · doi:10.1016/j.joule.2021.05.005 · Cited by 1,284
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Recent Advances and Prospective in Ruthenium-Based Materials for Electrochemical Water Splitting
Yu, J., He, Q., Yang, G., Zhou, W., Shao, Z., & Ni, M. (2019) · ACS Catalysis · doi:10.1021/acscatal.9b02457 · Cited by 789
Shan, J., Ling, T., Davey, K., Zheng, Y., & Qiao, S. (2019) · Advanced Materials · doi:10.1002/adma.201900510 · Cited by 642
Self-citationChen, S., Huang, H., Jiang, P., Yang, K., Diao, J., Gong, S., Liu, S., Huang, M., Wang, H., & Chen, Q. (2020) · ACS Catalysis · doi:10.1021/acscatal.9b04922 · Cited by 574
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Metadata
- Authors
- Shan, J., Guo, C., Zhu, Y., Chen, S., Song, L., Jaroniec, M., Zheng, Y., & Qiao, S.-Z.
- Venue
- Chem
- Publisher
- Elsevier BV
- Published
- 2019-02
- Volume
- 5
- Issue
- 2
- Pages
- 445-459
- ISSN
- 2451-9294 (ISSN-L)
- OpenAlex
- W2905737950
- Cited by
- 545
- References
- 14
- FWCI
- 10.01
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Shan, J., Guo, C., Zhu, Y., Chen, S., Song, L., Jaroniec, M., Zheng, Y., & Qiao, S.-Z. (2019). Charge-Redistribution-Enhanced Nanocrystalline Ru@IrOx Electrocatalysts for Oxygen Evolution in Acidic Media. Chem. https://doi.org/10.1016/j.chempr.2018.11.010
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