The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Efficient and Selective CO2 Reduction Integrated with Organic Synthesis by Solar Energy
Open accessAbstract
Summary Solar-driven catalytic CO2 reduction is attractive to produce usable fuels and value-added chemicals. However, conventional strategies suffer from low activity and/or expense of sacrificial reagents. Here, we describe the first example of CO2 reduction integrated with the oxidative organic synthesis by solar energy. With visible-light irradiation, CdSe/CdS quantum dots (QDs) enable photocatalytic conversion of CO2 to CO with an exciting rate of ∼412.8 mmol g−1 h−1 and a high selectivity of > 96% in the presence of triethylamine. More importantly, CO2-to-CO conversion proceeds smoothly when integrated with oxidative coupling of 1-phenylethanol to evolve pinacol. 1-Phenylethanol with electron-donating groups at the p-position of aryl ring, for example, is converted to corresponding pinacols with excellent yields up to 98%. The released protons and electrons of oxidative half-reaction are used for CO2 reduction. Apparently, this strategy provides the exact answer toward cost-effective CO2 photoreduction and opens a new horizon for efficient solar-to-fuel conversion.
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Cites
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Xu, H.-Q., Hu, J., Wang, D., Li, Z., Zhang, Q., Luo, Y., Yu, S.-H., & Jiang, H.-L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b08773 · Cited by 1,166
Cited by
Semiconductor Quantum Dots: An Emerging Candidate for CO2 Photoreduction
Wu, H., Li, X., Tung, C., & Wu, L. (2019) · Advanced Materials · doi:10.1002/adma.201900709 · Cited by 486
Self-citationYuan, L., Qi, M., Tang, Z., & Xu, Y. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202101667 · Cited by 375
Li, Q., Jiao, Y., Tang, Y., Zhou, J., Wu, B., Jiang, B., & Fu, H. (2023) · Journal of the American Chemical Society · doi:10.1021/jacs.3c05234 · Cited by 339
Highly active deficient ternary sulfide photoanode for photoelectrochemical water splitting
Wang, H., Xia, Y., Li, H., Wang, X., Yu, Y., Jiao, X., & Chen, D. (2020) · Nature Communications · doi:10.1038/s41467-020-16800-w · Cited by 283
Qi, M.-Y., Li, Y.-H., Anpo, M., Tang, Z.-R., & Xu, Y.-J. (2020) · ACS Catalysis · doi:10.1021/acscatal.0c04237 · Cited by 268
Metadata
- Authors
- Guo, Q., Liang, F., Li, X.-B., Gao, Y.-J., Huang, M.-Y., Wang, Y., Xia, S.-G., Gao, X.-Y., Gan, Q.-C., Lin, Z.-S., Tung, C.-H., & Wu, L.-Z.
- Venue
- Chem
- Publisher
- Elsevier BV
- Published
- 2019-10
- Volume
- 5
- Issue
- 10
- Pages
- 2605-2616
- ISSN
- 2451-9294 (ISSN-L)
- OpenAlex
- W2963775476
- Cited by
- 273
- References
- 2
- FWCI
- 6.54
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Guo, Q., Liang, F., Li, X.-B., Gao, Y.-J., Huang, M.-Y., Wang, Y., Xia, S.-G., Gao, X.-Y., Gan, Q.-C., Lin, Z.-S., Tung, C.-H., & Wu, L.-Z. (2019). Efficient and Selective CO2 Reduction Integrated with Organic Synthesis by Solar Energy. Chem. https://doi.org/10.1016/j.chempr.2019.06.019
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