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Organic-Inorganic-Induced Polymer Intercalation into Layered Composites for Aqueous Zinc-Ion Battery
Open accessAbstract
Summary Rechargeable aqueous zinc-based batteries are very attractive alternative devices for current energy storage by virtue of their low cost and high security. However, the performance of vanadium oxide cathode strongly relies on the distance of interlayer spacing. Here, we employ layered PEDOT-NH4V3O8 (PEDOT-NVO) as a cathode material, which produces an enlarged interlayer spacing of 10.8 A (against 7.8 A for the single NVO) by effectively conducting polymer intercalation. This cathode material exhibits an improved capacity of 356.8 mAh g−1 at 0.05 A g−1 and 163.6 mAh g−1, even at the highest current density of 10 A g−1 (with a high retention from 0.05 to 10 A g−1), and features an ultra-long lifetime of over 5,000 charge-discharge cycles with a capacity retention of 94.1%. A combination of mechanism analyses and theoretical calculations suggest that the oxygen vacancies and larger interlayer spacing through polymer assistance account for the improved electrochemical performance.
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Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Cited by
Li, M., Li, Z., Wang, X., Meng, J., Liu, X., Wu, B., Han, C., & Mai, L. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00030f · Cited by 559
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
Rechargeable aqueous zinc-ion batteries: Mechanism, design strategies and future perspectives
Liu, H., Wang, J.-G., You, Z., Wei, C., Kang, F., & Wei, B. (2021) · Materials Today · doi:10.1016/j.mattod.2020.08.021 · Cited by 282
Biomass‐Derived Carbon for High‐Performance Batteries: From Structure to Properties
Sun, Y., Shi, X., Yang, Y., Suo, G., Zhang, L., Lu, S., & Chen, Z. (2022) · Advanced Functional Materials · doi:10.1002/adfm.202201584 · Cited by 253
Metadata
- Authors
- Bin, D., Huo, W., Yuan, Y., Huang, J., Liu, Y., Zhang, Y., Dong, F., Wang, Y., & Xia, Y.
- Venue
- Chem
- Publisher
- Elsevier BV
- Published
- 2020-04
- Volume
- 6
- Issue
- 4
- Pages
- 968-984
- ISSN
- 2451-9294 (ISSN-L)
- OpenAlex
- W3007977033
- Cited by
- 424
- References
- 1
- FWCI
- 22.20
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Bin, D., Huo, W., Yuan, Y., Huang, J., Liu, Y., Zhang, Y., Dong, F., Wang, Y., & Xia, Y. (2020). Organic-Inorganic-Induced Polymer Intercalation into Layered Composites for Aqueous Zinc-Ion Battery. Chem. https://doi.org/10.1016/j.chempr.2020.02.001
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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