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Water reactivity in the liquid and supercritical CO2 phase: Has half the story been neglected?
Open accessAbstract
Aqueous-phase mediated chemical reactions with dissolved CO2 have long been considered the principal if not only reactive process supporting mineralization reactions with basalt and other reactive reservoir rocks and caprocks in deep geologic sequestration systems. This is not surprising given the quite high solubility of CO2 in the aqueous phase and ample evidence from natural systems of the reactivity of CO2charged waters with a variety of silicate minerals. In contrast, comparatively scant attention has been directed at reactivity of water solvated in liquid and supercritical CO2, with the exception of interest in the impacts of water in CO2 on the corrosion of pipeline steels. The results presented in this paper show that the most interesting and important aspects of water reactivity with metal and oxide surfaces of interest in geologic sequestration systems actually occurs in the liquid or supercritical CO2 phase.
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Cites
Spycher, N., Pruess, K., & Ennis-King, J. (2003) · Geochimica et Cosmochimica Acta · doi:10.1016/s0016-7037(03)00273-4 · Cited by 991
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Gaus, I. (2010) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2009.09.015 · Cited by 693
Comprehensive Review of Caprock-Sealing Mechanisms for Geologic Carbon Sequestration
Song, J., & Zhang, D. (2013) · Environmental Science & Technology · doi:10.1021/es301610p · Cited by 388
Carbon mineralization and geological storage of CO2 in basalt: Mechanisms and technical challenges
Raza, A., Glatz, G., Gholami, R., Mahmoud, M., & Alafnan, S. (2022) · Earth-Science Reviews · doi:10.1016/j.earscirev.2022.104036 · Cited by 328
Mineralization of carbon dioxide: A literature review
Romanov, V., Soong, Y., Carney, C., Rush, G. E., Nielsen, B., & O'Connor, W. (2015) · ChemBioEng Reviews · doi:10.1002/cben.201500002 · Cited by 262
Determining the corrosive potential of CO2 transport pipeline in high pCO2–water environments
Choi, Y.-S., & Nešić, S. (2011) · International Journal of Greenhouse Gas Control · doi:10.1016/j.ijggc.2010.11.008 · Cited by 256
Metadata
- Authors
- McGrail, B. P., Schaef, H. T., Glezakou, V.-A., Dang, L. X., & Owen, A. T.
- Venue
- Energy Procedia
- Publisher
- Elsevier BV
- Published
- 2009-02
- Volume
- 1
- Issue
- 1
- Pages
- 3415-3419
- ISSN
- 1876-6102 (ISSN-L)
- OpenAlex
- W2042071946
- Cited by
- 199
- References
- 1
- FWCI
- 27.40
- Type
- conference paper
- Language
- en
- Open access
- diamond
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- McGrail, B. P., Schaef, H. T., Glezakou, V.-A., Dang, L. X., & Owen, A. T. (2009). Water reactivity in the liquid and supercritical CO2 phase: Has half the story been neglected? Energy Procedia. https://doi.org/10.1016/j.egypro.2009.02.131
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
