Influence of dilute feed and pH on electrochemical reduction of CO2 to CO on Ag in a continuous flow electrolyzer
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Singh et al. claimed that larger cations provide stronger buffering abilities, maintain a lower pH and keep the local dissolved CO2 concentration higher.
“Alternatively, Singh et al. have recently claimed that larger cations provide stronger buffering abilities, maintain a lower pH and keep the local dissolved CO2 concentration higher (Figure .11).”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [215]
Higher CO2 concentrations reduce polarization losses, which preferentially improves selectivity towards C2H4 over CH4 and H2.
“The higher CO2 concentrations reduce polarization losses, which preferentially improves selectivity towards C2H4 over CH4 and H2.[215]”
From Electrochemical CO <sub>2</sub> Reduction into Chemical Feedstocks: From Mechanistic Electrocatalysis Models to System Design (2019) · cites this paper as [215]
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References 37 · Cited by 243
- Authors
- Kim, B., Ma, S., Molly Jhong, H.-R., & Kenis, P. J. A.
- Affiliations
- Kyushu University (JP)
- Corresponding author
- Kenis, Paul J.A.
- Venue
- Electrochimica Acta
- Publisher
- Elsevier BV
- Published
- 2015-06
- Volume
- 166
- Pages
- 271-276
- ISSN
- 0013-4686 (ISSN-L)
- OpenAlex
- W2034080509
- Cited by
- 243
- References
- 37
- Citations by year
- 2026: 24 · 2025: 24 · 2024: 36 · 2023: 21 · 2022: 23 · 2021: 24 · 2020: 26 · 2019: 22 · 2018: 19 · 2017: 9 · 2016: 14 · 2015: 1
- FWCI
- 4.24
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- Locations
- Electrochimica Acta (acceptedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- University of Illinois at Urbana-Champaign (DE-SC0004453)
- Ministry of Education, Culture, Sports, Science and Technology
- International Institute for Carbon-Neutral Energy Research, Kyushu University (WPI-I2CNER)
- U.S. Department of Energy
- National Science Foundation (CTS 05-47617)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Physical Sciences › Chemical Engineering › Catalysis › Catalysts for Methane Reforming
- Physical Sciences › Chemical Engineering › Process Chemistry and Technology › Carbon dioxide utilization in catalysis
- Keywords
- electrochemical CO2 reduction, CO2 to CO conversion, gas diffusion electrode, silver catalysts, pH effect, alkaline electrolyte, Faradaic efficiency, product selectivity, renewable energy utilization
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