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Chemical stability and long-term cell performance of low-cobalt, Ni-Rich cathodes prepared by aqueous processing for high-energy Li-Ion batteries
Open accessAbstract
Cobalt content in Li-ion battery cathodes has become a top concern due to its price volatility and limited source availability. Low-cobalt, Ni-rich active materials are promising candidates for next-generation cathodes due to their high capacities, and water-based processing of these materials can further reduce both cost and environmental impact. We systematically evaluated the water compatibility of four different LiNixMn1-x-yCoyO2 (NMC) powders with increasing nickel contents. Comprehensive characterization verified there is no major change to their bulk structures, and only slight surface modifications related to the removal of contaminant species. For the first time, we demonstrate that LiNi0.8Mn0.1Co0.1O2 (NMC 811) cathodes can be formulated in water and cycled 1000 times in full pouch cells with excellent capacity retention (~70% compared to ~76% for NMP-processed cells). When implemented in future battery production lines, aqueous processing of Ni-rich NMC will simultaneously enable cost reductions and higher cell energy densities.
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The development and future of lithium ion batteries
Blomgren, G. E. (2017) · Journal of The Electrochemical Society · doi:10.1149/2.0251701jes · Cited by 1,940
Cited by
Li, J., Fleetwood, J., Hawley, W. B., & Kays, W. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00565 · Cited by 895
Self-citationMao, J., Ye, C., Zhang, S., Xie, F., Zeng, R., Davey, K., Guo, Z., & Qiao, S. (2022) · Energy & Environmental Science · doi:10.1039/d2ee00162d · Cited by 365
Metadata
- Authors
- Wood, M., Li, J., Ruther, R. E., Du, Z., Self, E. C., Meyer, H. M., Daniel, C., Belharouak, I., & Wood, D. L.
- Venue
- Energy Storage Materials
- Publisher
- Elsevier BV
- Published
- 2020-01
- Volume
- 24
- Pages
- 188-197
- ISSN
- 2405-8289 (ISSN-L)
- 2405-8297
- OpenAlex
- W2970178053
- Cited by
- 237
- References
- 1
- FWCI
- 10.84
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- CoChat. (2026). Citation check: Chemical stability and long-term cell performance of low-cobalt, Ni-Rich cathodes prepared by aqueous processing for high-energy Li-Ion batteries. https://app.cochat.ai/papers/10.1016/j.ensm.2019.08.020
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- Wood, M., Li, J., Ruther, R. E., Du, Z., Self, E. C., Meyer, H. M., Daniel, C., Belharouak, I., & Wood, D. L. (2020). Chemical stability and long-term cell performance of low-cobalt, Ni-Rich cathodes prepared by aqueous processing for high-energy Li-Ion batteries. Energy Storage Materials. https://doi.org/10.1016/j.ensm.2019.08.020
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