Expanding the low-temperature and high-voltage limits of aqueous lithium-ion battery
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The water/DOL hybrid electrolyte displays a stable electrochemical window of 4.7 V, attributed to reduced content of free water molecules at the anode surface, leading to robust LiF-rich SEI formation that substantially suppresses hydrogen evolution.
“The water/DOL hybrid electrolyte displays a stable electrochemical window of 4.7 V, which is attributed to the reduced content of the free water molecules at the anode surface, leading to robust LiF-rich SEI formation that substantially suppresses hydrogen evolution.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [85]
At low temperatures, the remaining liquid phase predominantly consists of the Li+-DOL solvation complex, whose weak binding energy benefits the Li+ desolvation process at the electrode, as evidenced by the low activation energy barrier and high exchange current density for Li+ de/intercalation.
“At LTs, the remaining liquid phase predominantly consists of the Li + -DOL solvation complex, whose weak binding energy benefits the Li + desolvation process at the electrode, as evidenced by the low activation energy barrier and the high exchange current density for Li + de/intercalation to electrodes.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [85]
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References 37 · Cited by 142
- Authors
- Ma, Z., Chen, J., Vatamanu, J., Borodin, O., Bedrov, D., Zhou, X., Zhang, W., Li, W., Xu, K., & Xing, L.
- Affiliations
- South China Normal University (CN)
- DEVCOM Army Research Laboratory (US)
- University of Utah (US)
- Corresponding author
- Xu, Kang
- Xing, Lidan
- ORCID
- Venue
- Energy Storage Materials
- Publisher
- Elsevier BV
- Published
- 2022-03
- Volume
- 45
- Pages
- 903-910
- ISSN
- 2405-8289 (ISSN-L)
- 2405-8297
- OpenAlex
- W4200377154
- Cited by
- 142
- References
- 37
- Citations by year
- 2026: 23 · 2025: 32 · 2024: 34 · 2023: 39 · 2022: 14
- FWCI
- 6.40
- Type
- journal article
- Language
- en
- Open access
- bronze
- doi.org
- Licence
- www.elsevier.com/tdm/userlicense/1.0/ (tdm)
- www.elsevier.com/legal/tdmrep-license (tdm)
- www.elsevier.com/open-access/userlicense/1.0/ (am, 309 d)
- doi.org/10.15223/policy-017 (stm-asf)
- doi.org/10.15223/policy-037 (stm-asf)
- doi.org/10.15223/policy-012 (stm-asf)
- doi.org/10.15223/policy-029 (stm-asf)
- doi.org/10.15223/policy-004 (stm-asf)
- Locations
- Energy storage materials (acceptedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- Funders
- National Natural Science Foundation of China (21573080)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced battery technologies research
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Keywords
- aqueous lithium-ion batteries, 1,3-dioxolane, hybrid electrolytes, electrochemical stability window, low-temperature operation, fast ion transport, LiF-rich interphase, Li+ desolvation, LiMn2O4 cathode, Li4Ti5O12 anode, Coulombic efficiency, non-flammable electrolytes
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