The DOI matches its Crossref record; 350 of the 350 references it cites were found in a registry or an index.
Top-down synthesis of graphene: A comprehensive review
Abstract
Abstract Graphene research has become an emerging frontier in materials science because of its potential as a versatile material in multiple applications, from electronics, sensors, water treatment, batteries, displays, advanced composites, and coatings to biomedical applications. While the community has witnessed tremendous advances in the laboratory-scale synthesis of graphene, it is crucial to focus on sustainable large-scale graphene production to adopt graphene-based technology at an industrial scale. Several top-down and bottom-up methods have been developed to realize affordable graphene production. However, a low-cost scalable graphene production method with acceptable quality remains a challenge; top-down processes are demonstrating their potential to offer a more straightforward solution. Herein, we present an overview of recent progress in the research and development of top-down graphene synthesis methods and their potential to scale-up graphene production. We cover the effect of different synthesis parameters on the quality control of graphene. In addition, we provide a brief overview of bottom-up methods. Finally, we discuss the existing challenges and future directions in top-down methods for large-scale graphene production.
Overview
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Integrity signals
Registry
Cites
Statistics
Verification
Claims the paper makes
The claims and statistics of this paper haven’t been checked yet.
Run the check — free, no account needed. It reads the open-access text and checks the sources it cites.
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
The self-check needs the paper’s full text.
Citations
Cites
Electric Field Effect in Atomically Thin Carbon Films
Novoselov, K. S., Geim, A. K., Morozov, S. V., Jiang, D., Zhang, Y., Dubonos, S. V., Grigorieva, I. V., & Firsov, A. A. (2004) · Science · doi:10.1126/science.1102896 · Cited by 66,834
Preparation of Graphitic Oxide
Hummers, W. S., & Offeman, R. E. (1958) · Journal of the American Chemical Society · doi:10.1021/ja01539a017 · Cited by 29,920
Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide
Stankovich, S., Dikin, D. A., Piner, R. D., Kohlhaas, K. A., Kleinhammes, A., Jia, Y., Wu, Y., Nguyen, S. T., & Ruoff, R. S. (2007) · Carbon · doi:10.1016/j.carbon.2007.02.034 · Cited by 13,878
Improved Synthesis of Graphene Oxide
Marcano, D. C., Kosynkin, D. V., Berlin, J. M., Sinitskii, A., Sun, Z., Slesarev, A., Alemany, L. B., Lu, W., & Tour, J. M. (2010) · ACS Nano · doi:10.1021/nn1006368 · Cited by 11,989
The chemistry of graphene oxide
Dreyer, D. R., Park, S., Bielawski, C. W., & Ruoff, R. S. (2010) · Chem. Soc. Rev. · doi:10.1039/b917103g · Cited by 11,653
Large-Area Synthesis of High-Quality and Uniform Graphene Films on Copper Foils
Li, X., Cai, W., An, J., Kim, S., Nah, J., Yang, D., Piner, R., Velamakanni, A., Jung, I., Tutuc, E., et al. (2009) · Science · doi:10.1126/science.1171245 · Cited by 11,220
Novoselov, K. S., Fal′ko, V. I., Colombo, L., Gellert, P. R., Schwab, M. G., & Kim, K. (2012) · Nature · doi:10.1038/nature11458 · Cited by 9,251
Unconventional superconductivity in magic-angle graphene superlattices
Cao, Y., Fatemi, V., Fang, S., Watanabe, K., Taniguchi, T., Kaxiras, E., & Jarillo-Herrero, P. (2018) · Nature · doi:10.1038/nature26160 · Cited by 8,300
Roll-to-roll production of 30-inch graphene films for transparent electrodes
Bae, S., Kim, H., Lee, Y., Xu, X., Park, J.-S., Zheng, Y., Balakrishnan, J., Lei, T., Ri Kim, H., Song, Y. I., et al. (2010) · Nature Nanotechnology · doi:10.1038/nnano.2010.132 · Cited by 8,136
Solid C60: a new form of carbon
Krätschmer, W., Lamb, L. D., Fostiropoulos, K., & Huffman, D. R. (1990) · Nature · doi:10.1038/347354a0 · Cited by 7,646
Metadata
- Authors
- Kumar, N., Salehiyan, R., Chauke, V., Joseph Botlhoko, O., Setshedi, K., Scriba, M., Masukume, M., & Sinha Ray, S.
- Venue
- FlatChem
- Publisher
- Elsevier BV
- Published
- 2021-05
- Volume
- 27
- Pages
- 100224
- ISSN
- 2452-2627 (ISSN-L)
- OpenAlex
- W3128629069
- Cited by
- 336
- References
- 350
- FWCI
- 16.42
- Type
- journal article
- Language
- en
- Open access
- closed
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
Are you an author, or do you see a problem with this page? Request a review
How to cite
Cite CoChat for the checks on this page, and the paper for its own findings.
- This page
- CoChat. (2026). Citation check: Top-down synthesis of graphene: A comprehensive review. https://app.cochat.ai/papers/10.1016/j.flatc.2021.100224
- The paper
- Kumar, N., Salehiyan, R., Chauke, V., Joseph Botlhoko, O., Setshedi, K., Scriba, M., Masukume, M., & Sinha Ray, S. (2021). Top-down synthesis of graphene: A comprehensive review. FlatChem. https://doi.org/10.1016/j.flatc.2021.100224
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.