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Sustainable hierarchical porous carbon aerogel from cellulose for high-performance supercapacitor and CO2 capture
Abstract
Fabrication of cost-effective and eco-friendly hierarchical porous carbons from the most abundant and widely available biomass cellulose represents a critical and sustainable way to solve the crisis of fossil resources. In this work, a hierarchical porous carbon aerogel with desirable macropores, mesopores, and micropores was obtained via dissolving-gelling and subsequent carbonizing-activating process. The CO2 activated carbon aerogel had a high specific surface area of 1364m2/g and a high specific capacitance of 328Fg−1 (0.5Ag−1, 1.0M H2SO4) as well as an outstanding cycling stability with 96% of the capacitance retention after 5000 charge/discharge cycles. More importantly, for the first time, we demonstrated that the cellulose-derived hierarchical porous carbon aerogel showed a good CO2 adsorption capacity of 3.42mmol/g (at 1atm and 298K), which indicates the possibility of using this carbon aerogel for CO2 capture.
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“biomass (e.g., cellulose, 17 chitosan, 18 lignin, 19,20 and biomass waste.21 ) has emerged as an important class of precursors for carbon aerogel fabrication, offering abundant, renewable, environmentally friendly, and cost-effective resources.”
From Boosting hydrogen production with raspberry-derived carbon aerogels with in situ grown carbon nanotubes (2026) · cites this paper as [17]
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Metadata
- Authors
- Zhuo, H., Hu, Y., Tong, X., Zhong, L., Peng, X., & Sun, R.
- Affiliations
- State Key Laboratory of Pulp and Paper Engineering (CN)
- Corresponding author
- Zhong, Linxin
- Peng, Xinwen
- Venue
- Industrial Crops and Products
- Publisher
- Elsevier BV
- Published
- 2016-09
- Volume
- 87
- Pages
- 229-235
- ISSN
- 0926-6690 (ISSN-L)
- OpenAlex
- W2344089845
- Cited by
- 196
- References
- 34
- Citations by year
- 2026: 8 · 2025: 14 · 2024: 21 · 2023: 22 · 2022: 26 · 2021: 25 · 2020: 19 · 2019: 24 · 2018: 22 · 2017: 11 · 2016: 4
- FWCI
- 6.39
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Industrial Crops and Products (publishedVersion)
- Funders
- National Natural Science Foundation of China (21506068)
- State Key Laboratory of Pulp and Paper Engineering (2015ZD03, 2015QN05)
- Pearl River S&T Nova Program of Guangzhou
- Guangdong natural Science Foundation (2014A030310319)
- Science and Technology Program of Guangzhou (201504010033)
- Major State Basic Research Projects of China (973-2012CB215302)
- Fundamental Research Funds for the Central Universities
- Topics
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
- Physical Sciences › Materials Science › Biomaterials › Advanced Cellulose Research Studies
- Keywords
- cellulose, biomass-derived carbon, supercapacitor electrodes, CO2 adsorption, CO2 capture, specific capacitance, cycling stability, carbonization and activation
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