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Treatment of wastewater containing methyl orange dye by fluidized three dimensional electrochemical oxidation process integrated with chemical oxidation and adsorption
Abstract
The integrated high-efficiency treatment technology for dye industry wastewater is one of the current research hot topic in industrial wastewater treatment area. This article reports a new fluidized three-dimensional electrochemical treatment process integrating activated carbon adsorption, direct electro-oxidation and ·OH oxidation. In the process, activated carbon is polarized in a fluidized bed electrochemical reactor to enhance the direct electro-oxidation and ·OH oxidation, and there is a synergistic effect of effective adsorption and electrochemical oxidation to strengthen the treatment efficiency. When 200 mg/L methyl orange is processed, its removal rate reaches 99.9% in 30min, and the synergistic efficiency is 57.3%. After 8 cycles of activated carbon reusage in the process, the removal rate of methyl orange still kept at 89.2%. It is also founded that the activated carbon maintains 64.5% of its original adsorption capacity during the cycle. These results shows its interesting application potential in the fields of high-efficiency, low-cost and green treatment of various industrial organic wastewaters. Further improvements should focus on the development of continuous operation model and the improvement of the activated carbon electro-catalytic performance and the practical regeneration ways of the activated carbon particle electrodes.
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Metadata
- Authors
- Liu, X., Chen, Z., Du, W., Liu, P., Zhang, L., & Shi, F.
- Affiliations
- Changchun University of Technology (CN)
- Corresponding author
- Zhang, Long
- Shi, Fengwei
- Venue
- Journal of Environmental Management
- Publisher
- Elsevier BV
- Published
- 2022-06
- Volume
- 311
- Pages
- 114775
- ISSN
- 0301-4797 (ISSN-L)
- OpenAlex
- W4214603813
- Cited by
- 124
- References
- 48
- Citations by year
- 2026: 29 · 2025: 19 · 2024: 31 · 2023: 24 · 2022: 21
- FWCI
- 7.06
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Locations
- Journal of Environmental Management (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
- Physical Sciences › Environmental Science › Water Science and Technology › Coagulation and Flocculation Studies
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Keywords
- methyl orange, dye wastewater treatment, three-dimensional electrodes, activated carbon adsorption, hydroxyl radical oxidation, chemical oxidation, activated carbon regeneration, dye removal, electrocatalysis
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