Mineral carbonation for carbon sequestration in cement kiln dust from waste piles
Abstract
Alkaline earth metals, such as calcium and magnesium oxides, readily react with carbon dioxide (CO(2)) to produce stable carbonate minerals. Carbon sequestration through the formation of carbonate minerals is a potential means to reduce CO(2) emissions. Calcium-rich, industrial solid wastes and residues provide a potential source of highly reactive oxides, without the need for pre-processing. This paper presents the first study examining the feasibility of carbon sequestration in cement kiln dust (CKD), a byproduct generated during the manufacturing of cement. A series of column experiments were conducted on segments of intact core taken from landfilled CKD. Based on stoichiometry and measured consumption of CO(2) during the experiments, degrees of carbonation greater than 70% of the material's potential theoretical extent were achieved under ambient temperature and pressure conditions. The overall extent of carbonation/sequestration was greater in columns with lower water contents. The major sequestration product appears to be calcite; however, more detailed material characterization is need on pre- and post-carbonated samples to better elucidate carbonation pathways and products.
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The CO2 uptake capacity of waste gypsum was estimated between 11% and 25%.
“the CO 2 uptake capacity of waste gypsum and cement kiln dust was estimated between 11% and 25% and between 8.68% and 11.68%, respectively.”
From An overview of utilizing CO2 for accelerated carbonation treatment in the concrete industry (2022) · cites this paper as [63]
The CO2 uptake capacity of cement kiln dust was estimated between 8.68% and 11.68%.
“the CO 2 uptake capacity of waste gypsum and cement kiln dust was estimated between 11% and 25% and between 8.68% and 11.68%, respectively.”
From An overview of utilizing CO2 for accelerated carbonation treatment in the concrete industry (2022) · cites this paper as [63]
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- Authors
- Huntzinger, D. N., Gierke, J. S., Sutter, L. L., Kawatra, S. K., & Eisele, T. C.
- Affiliations
- University of Michigan (US)
- Michigan Technological University (US)
- Corresponding author
- Huntzinger, Deborah N.
- Venue
- Journal of Hazardous Materials
- Publisher
- Elsevier BV
- Published
- 2009-08-30
- Volume
- 168
- Issue
- 1
- Pages
- 31-37
- ISSN
- 0304-3894 (ISSN-L)
- OpenAlex
- W2128180942
- Cited by
- 217
- References
- 4
- Citations by year
- 2026: 16 · 2025: 21 · 2024: 24 · 2023: 12 · 2022: 15 · 2021: 15 · 2020: 13 · 2019: 11 · 2018: 14 · 2017: 13 · 2016: 10 · 2015: 10 · 2014: 6 · 2013: 10 · 2012: 11
- FWCI
- 7.47
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Hazardous Materials (publishedVersion)
- PubMed (publishedVersion)
- Digital Commons - Michigan Tech (Michigan Technological University) (submittedVersion)
- Funders
- National Science Foundation
- Iowa State University
- National Energy Technology Laboratory
- Division of Graduate Education
- Topics
- Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
- Physical Sciences › Engineering › Civil and Structural Engineering › Concrete and Cement Materials Research
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Keywords
- CO2 mineralization, carbon sequestration, cement kiln dust, CO2 emission reduction, calcite formation, alkaline earth oxides, industrial waste landfill, column experiments, water content effects, carbonation degree
- MeSH terms
- Carbon, Carbon Dioxide, Construction Materials, Industrial Waste, Manufactured Materials, Minerals, Environmental Restoration and Remediation
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