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Phase Transition Control for High-Performance Blade-Coated Perovskite Solar Cells
Open accessAbstract
Summary Here, we have identified that the key issue for rational transitioning from spin-coating to blade-coating processes of perovskite films arises from whether intermediate phases participate in the phase transition. In situ characterizations were carried out to provide a comprehensive picture of structural evolution and crystal growth mechanisms. These findings present opportunities for designing an effective process for blade-coating perovskite film: a large-grained dense perovskite film with high crystal quality and photophysical properties can be obtained only via direct crystallization for both spin-coating and blade-coating processes. As a result, the blade-coated MAPbI3 films deliver excellent charge-collection efficiency at both short circuit and open circuit, and photovoltaic properties with efficiencies of 18.74% (0.09 cm2) and 17.06% (1 cm2) in planar solar cells. The significant advances in understanding how the phase transition links spin-coating and blade-coating processes should provide a path toward high-performance printed perovskite devices.
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Cites
Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
Jeon, N. J., Noh, J. H., Kim, Y. C., Yang, W. S., Ryu, S., & Seok, S. I. (2014) · Nature Materials · doi:10.1038/nmat4014 · Cited by 6,723
120 mm single-crystalline perovskite and wafers: towards viable applications
Liu, Y., Ren, X., Zhang, J., Yang, Z., Yang, D., Yu, F., Sun, J., Zhao, C., Yao, Z., Wang, B., et al. (2017) · Science China Chemistry · doi:10.1007/s11426-017-9081-3 · Cited by 144
Self-citation
Cited by
Understanding of perovskite crystal growth and film formation in scalable deposition processes
Liu, C., Cheng, Y.-B., & Ge, Z. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00711c · Cited by 675
From scalable solution fabrication of perovskite films towards commercialization of solar cells
Huang, F., Li, M., Siffalovic, P., Cao, G., & Tian, J. (2019) · Energy & Environmental Science · doi:10.1039/c8ee03025a · Cited by 351
Niu, T., Zhu, W., Zhang, Y., Xue, Q., Jiao, X., Wang, Z., Xie, Y.-M., Li, P., Chen, R., Huang, F., et al. (2021) · Joule · doi:10.1016/j.joule.2020.12.003 · Cited by 320
Self-citationMaterials and Methods for High‐Efficiency Perovskite Solar Modules
Lee, D.-K., & Park, N.-G. (2022) · Solar RRL · doi:10.1002/solr.202100455 · Cited by 86
Mundt, L. E., & Schelhas, L. T. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201903074 · Cited by 58
Metadata
- Authors
- Li, J., Munir, R., Fan, Y., Niu, T., Liu, Y., Zhong, Y., Yang, Z., Tian, Y., Liu, B., Sun, J., Smilgies, D.-M., Thoroddsen, S., Amassian, A., Zhao, K., & Liu, S. (.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2018-07
- Volume
- 2
- Issue
- 7
- Pages
- 1313-1330
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2802155296
- Cited by
- 260
- References
- 2
- FWCI
- 11.29
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Li, J., Munir, R., Fan, Y., Niu, T., Liu, Y., Zhong, Y., Yang, Z., Tian, Y., Liu, B., Sun, J., Smilgies, D.-M., Thoroddsen, S., Amassian, A., Zhao, K., & Liu, S. (. (2018). Phase Transition Control for High-Performance Blade-Coated Perovskite Solar Cells. Joule. https://doi.org/10.1016/j.joule.2018.04.011
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