The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Enabling High-Voltage Lithium-Metal Batteries under Practical Conditions
Open accessAbstract
Summary Rechargeable lithium (Li)-metal batteries (LMBs) offer a great opportunity for applications needing high-energy-density battery systems. However, rare progress has been demonstrated so far under practical conditions, including high voltage, high-loading cathode, thin Li anode, and lean electrolyte. Here, in opposition to common wisdom, we report an ether-based localized high-concentration electrolyte that can greatly enhance the stability of a Ni-rich LiNi0.8Mn0.1Co0.1O2 (NMC811) cathode under 4.4 and 4.5 V with an effective protection interphase enriched in LiF. This effect, in combination with the superior Li stability in this electrolyte, enables dramatically improved cycling performances of Li||NMC811 batteries under highly challenging conditions. The LMBs can retain over 80% capacity in 150 stable cycles with extremely limited amounts of the Li anode and electrolyte. The findings in this work point out a very promising strategy to develop practical high-energy LMBs.
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Cites
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Self-citationHigh rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Self-citationInterface Stability in Solid-State Batteries
Richards, W. D., Miara, L. J., Wang, Y., Kim, J. C., & Ceder, G. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b04082 · Cited by 1,652
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Rational solvent molecule tuning for high-performance lithium metal battery electrolytes
Yu, Z., Rudnicki, P. E., Zhang, Z., Huang, Z., Celik, H., Oyakhire, S. T., Chen, Y., Kong, X., Kim, S. C., Xiao, X., et al. (2022) · Nature Energy · doi:10.1038/s41560-021-00962-y · Cited by 937
Tailoring electrolyte solvation for Li metal batteries cycled at ultra-low temperature
Holoubek, J., Liu, H., Wu, Z., Yin, Y., Xing, X., Cai, G., Yu, S., Zhou, H., Pascal, T. A., Chen, Z., et al. (2021) · Nature Energy · doi:10.1038/s41560-021-00783-z · Cited by 851
Critical effects of electrolyte recipes for Li and Na metal batteries
Zheng, X., Huang, L., Ye, X., Zhang, J., Min, F., Luo, W., & Huang, Y. (2021) · Chem · doi:10.1016/j.chempr.2021.02.025 · Cited by 367
Self-citationHoloubek, J., Yu, M., Yu, S., Li, M., Wu, Z., Xia, D., Bhaladhare, P., Gonzalez, M. S., Pascal, T. A., Liu, P., et al. (2020) · ACS Energy Letters · doi:10.1021/acsenergylett.0c00643 · Cited by 351
Cao, Z., Zheng, X., Qu, Q., Huang, Y., & Zheng, H. (2021) · Advanced Materials · doi:10.1002/adma.202103178 · Cited by 336
Metadata
- Authors
- Ren, X., Zou, L., Cao, X., Engelhard, M. H., Liu, W., Burton, S. D., Lee, H., Niu, C., Matthews, B. E., Zhu, Z., Wang, C., Arey, B. W., Xiao, J., Liu, J., Zhang, J.-G., & Xu, W.
- Venue
- Joule
- Publisher
- Elsevier BV
- Published
- 2019-07
- Volume
- 3
- Issue
- 7
- Pages
- 1662-1676
- ISSN
- 2542-4351 (ISSN-L)
- OpenAlex
- W2949049758
- Cited by
- 1,092
- References
- 5
- FWCI
- 31.99
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Ren, X., Zou, L., Cao, X., Engelhard, M. H., Liu, W., Burton, S. D., Lee, H., Niu, C., Matthews, B. E., Zhu, Z., Wang, C., Arey, B. W., Xiao, J., Liu, J., Zhang, J.-G., & Xu, W. (2019). Enabling High-Voltage Lithium-Metal Batteries under Practical Conditions. Joule. https://doi.org/10.1016/j.joule.2019.05.006
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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