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Challenges and perspectives of garnet solid electrolytes for all solid-state lithium batteries

Liu, Qi, Geng, Zhen, Han, Cuiping, Fu, Yongzhu, Li, Song, He, Yan-bing, Kang, Feiyu, Li, Baohua·2018·Journal of Power Sources
DOI 10.1016/j.jpowsour.2018.04.019
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Abstract

Abstract Garnet Li7La3Zr2O12 (LLZO) solid electrolytes recently have attracted tremendous interest as they have the potential to enable all solid-state lithium batteries (ASSLBs) owing to high ionic conductivity (10−3 to 10−4 S cm−1), negligible electronic transport, wide potential window (up to 9 V), and good chemical stability. Here we present the key issues and challenges of LLZO in the aspects of ion conduction property, interfacial compatibility, and stability in air. First, different preparation methods of LLZO are reviewed. Then, recent progress about the improvement of ionic conductivity and interfacial property between LLZO and electrodes are presented. Finally, we list some emerging LLZO-based solid-state batteries and provide perspectives for further research. The aim of this review is to summarize the up-to-date developments of LLZO and lead the direction for future development which could enable LLZO-based ASSLBs.

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Metadata

Authors
Liu, Q., Geng, Z., Han, C., Fu, Y., Li, S., He, Y.-B., Kang, F., & Li, B.
Venue
Journal of Power Sources
Publisher
Elsevier BV
Published
2018-06
Volume
389
Pages
120-134
ISSN
0378-7753 (ISSN-L)
DOI
10.1016/j.jpowsour.2018.04.019
OpenAlex
W2797994582
Cited by
478
References
98
FWCI
21.07
Type
journal article
Language
en
Open access
closed
Licence
  • www.elsevier.com/tdm/userlicense/1.0/ (tdm)
  • www.elsevier.com/legal/tdmrep-license (tdm)
Funders
  • Research Grants Council, University Grants Committee (T23-407/13-N)
  • National Natural Science Foundation of China (51232005, U1401243)
  • Shenzhen Technical Project (JCYJ20150529164918735, KQJSCX20160226191136, JCYJ20170412170911187)
  • National Key Research and Development Program of China (2014CB932400)
  • China Postdoctoral Science Foundation (2016 M601018)

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CoChat. (2026). Citation check: Challenges and perspectives of garnet solid electrolytes for all solid-state lithium batteries. https://app.cochat.ai/papers/10.1016/j.jpowsour.2018.04.019
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Liu, Q., Geng, Z., Han, C., Fu, Y., Li, S., He, Y.-B., Kang, F., & Li, B. (2018). Challenges and perspectives of garnet solid electrolytes for all solid-state lithium batteries. Journal of Power Sources. https://doi.org/10.1016/j.jpowsour.2018.04.019

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