Improving the graphite/electrolyte interface in lithium-ion battery for fast charging and low temperature operation: Fluorosulfonyl isocyanate as electrolyte additive
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Isocyanate-based additives can be electrochemically polymerized and form polyamide-like SEIs.
“It was reported that isocyanate-based additives can be electrochemically polymerized and form polyamide-like SEIs.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [128]
One problem of using FI as additive is low initial Coulombic efficiency, caused by Li consumption through SEI formation during the first cycle.
“One problem of using FI as additive is the low initial Coulombic efficiency, caused by the consumption of Li through SEI formation during the first cycle.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [128]
The FI-derived inorganic layer is mainly composed of LiF, ROSO2Li, Li2S, Li2SO3 and low concentrations of Li2CO3, Li2O and LixPFyOz, resulting in overall lower interface resistance.
“Although the inorganic layer was thicker by using FI, it is mainly composed of LiF, ROSO 2 Li, Li 2 S, Li 2 SO 3 and a low concentration of Li 2 CO 3 , Li 2 O and Li x PF y O z , resulting in overall lower interface resistance.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [128]
The thickness reduction of the organic species layer is attributed to suppression of carbonate solvent decomposition, while the increased thickness of the inorganic layer is attributed to FI-derived SEI components.
“The thickness reduction of the organic species layer was attributed to the suppression of carbonate solvent decomposition, while the increased thickness of the inorganic layer was attributed to the FI-derived SEI components.”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [128]
The SEI formed with FI additive is thicker, with thicker inorganic layers but thinner organic layers, compared to the SEI formed in conventional carbonate electrolytes without FI.
“They reported that compared with the SEI formed in conventional carbonate electrolytes without FI additive, the SEI formed in the electrolyte with FI additive was thicker, having thicker inorganic layers but thinner organic layers (Fig. 14c).”
From Review on Low-Temperature Electrolytes for Lithium-Ion and Lithium Metal Batteries (2023) · cites this paper as [128]
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“Till now, introducing these species in SEI by using electrolyte additives or highly concentrated electrolytes has been regarded as a successful strategy 26,27 .”
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“As a result, the detrimental interfacial reactions lead to the particle cracks, SEI growth, and electrolyte depletion, which deteriorate long‐term stability of LIBs.”
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“A similar combination of sulfur-based decomposition products has been reported by introducing fluorosulfonyl isocyanate (FI) to the EC-based electrolyte (LiPF6 in EC/DMC) and the improved performance of the SEI has been correlated with this modified composition (Shi et al., 2019).”
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“This effectively prevented the growth of an external organic layer and significantly decreased the resistance of the graphite/electrolyte interface [36].”
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“Among these, p-toluenesulfonyl isocyanate [17], 3-(phenylsulfonyl) propionitrile [18], fluorosulfonyl isocyanate [19], and, p-toluenesulfonyl methyl isocyanide [20] could be mentioned as examples which contain different nitrogen-based and sulfur-based groups in their molecular structures.”
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Synergistic Interfacial‐Bulk Solvation Enables Fast‐Charging and Low Temperature Li‐Ion Batteries
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- Authors
- Shi, J., Ehteshami, N., Ma, J., Zhang, H., Liu, H., Zhang, X., Li, J., & Paillard, E.
- Affiliations
- Forschungszentrum Jülich (DE)
- State Key Laboratory of Chemical Resource Engineering (CN)
- University of Münster (DE)
- Corresponding author
- Shi, Junli
- Zhang, Xin
- Paillard, Elie
- Venue
- Journal of Power Sources
- Publisher
- Elsevier BV
- Published
- 2019-07
- Volume
- 429
- Pages
- 67-74
- ISSN
- 0378-7753 (ISSN-L)
- OpenAlex
- W2944777829
- Cited by
- 147
- References
- 0
- Citations by year
- 2026: 17 · 2025: 11 · 2024: 24 · 2023: 25 · 2022: 22 · 2021: 30 · 2020: 18
- FWCI
- 6.29
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Power Sources (publishedVersion)
- Ningbo Institute of Materials Technology and Engineering, CAS Institutional Repository (submittedVersion)
- JuSER (Forschungszentrum Jülich) (submittedVersion)
- Virtual Community of Pathological Anatomy (University of Castilla La Mancha) (submittedVersion)
- Funders
- China Scholarship Council (CSC) ([2016]3035)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
- Physical Sciences › Engineering › Automotive Engineering › Advanced Battery Technologies Research
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
- Keywords
- solid electrolyte interphase, electrolyte additives, graphite anode, lithium-ion batteries, fast charging, low-temperature operation, interfacial resistance, rate capability
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