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Surface Defects in Two-Dimensional Photocatalysts for Efficient Organic Synthesis
Open accessAbstract
Summary Photocatalytic organic synthesis, utilizing economical and clean solar energy, can significantly decrease fossil energy consumption and environmental pollution but still suffers from low conversion efficiency and poor selectivity. Exploring advanced two-dimensional (2D) photocatalysts by introducing surface defects such as vacancy, functional modification, hybrid structure, and structural distortions are demonstrated to be effective strategies for increasing conversion efficiency and selectivity of relevant photocatalytic reactions. This review provides an overview of recent reports about the roles of surface defect engineering played on organic synthesis of 2D photocatalysts. In detail, a series of selective organic reactions and conversions of CO2 to valuable organic chemicals along with their corresponding mechanisms are presented, clarifying relationships between the introduced defects and photocatalytic performances of 2D photocatalysts. Finally, the difficulties and challenges as well as personal perspectives of possible solutions on designing advanced 2D photocatalysts by surface defect engineering for organic synthesis are proposed.
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Cites
Physical Mechanisms of Generation and Deactivation of Singlet Oxygen
Schweitzer, C., & Schmidt, R. (2003) · Chemical Reviews · doi:10.1021/cr010371d · Cited by 2,123
Partially oxidized atomic cobalt layers for carbon dioxide electroreduction to liquid fuel
Gao, S., Lin, Y., Jiao, X., Sun, Y., Luo, Q., Zhang, W., Li, D., Yang, J., & Xie, Y. (2016) · Nature · doi:10.1038/nature16455 · Cited by 1,865
Self-citation
Cited by
Zhang, X., Ma, P., Wang, C., Gan, L., Chen, X., Zhang, P., Wang, Y., Li, H., Wang, L., Zhou, X., et al. (2022) · Energy & Environmental Science · doi:10.1039/d1ee02369a · Cited by 909
Self-citationStrategies and Challenges on Selectivity of Photocatalytic Oxidation of Organic Substances
Xiong, L., & Tang, J. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202003216 · Cited by 530
ZnIn2S4‐Based Photocatalysts for Energy and Environmental Applications
Yang, R., Mei, L., Fan, Y., Zhang, Q., Zhu, R., Amal, R., Yin, Z., & Zeng, Z. (2021) · Small Methods · doi:10.1002/smtd.202100887 · Cited by 319
Zu, D., Ying, Y., Wei, Q., Xiong, P., Ahmed, M. S., Lin, Z., Li, M. M., Li, M., Xu, Z., Chen, G., et al. (2024) · Angewandte Chemie International Edition · doi:10.1002/anie.202405756 · Cited by 291
Defect engineering in nanozymes
Wu, Y., Xu, W., Jiao, L., Tang, Y., Chen, Y., Gu, W., & Zhu, C. (2022) · Materials Today · doi:10.1016/j.mattod.2021.10.032 · Cited by 269
Metadata
- Authors
- Sun, X., Zhang, X., & Xie, Y.
- Venue
- Matter
- Publisher
- Elsevier BV
- Published
- 2020-04
- Volume
- 2
- Issue
- 4
- Pages
- 842-861
- ISSN
- 2590-2385 (ISSN-L)
- OpenAlex
- W3014919922
- Cited by
- 182
- References
- 2
- FWCI
- 4.82
- Type
- journal article
- Language
- en
- Open access
- bronze
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