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Mesoporous CeO2 and CuO-loaded mesoporous CeO2: Synthesis, characterization, and CO catalytic oxidation property
Abstract
Abstract Mesoporous cerium dioxide has been synthesized using the ordered mesoporous silica KIT-6 as hard template. A series of different amounts of CuO have been modified to this CeO2 replica by wet impregnation. The XRD, SEM, TEM, N2 sorption measurement, and the CO catalytic oxidation reaction have been adopted to characterize those materials. CuO can be homogeneously loaded on this ceria replica. Compared with the porous CeO2 directly decomposed from the cerium nitrate hydrate, this CeO2 shows high catalytic reactivity for the CO oxidation, the T50 on this ceria replica is 83 K lower than on the decomposed ceria, and the CuO-loaded mesoporous ceria show more active for this catalytic reaction, the lowest T50 is only 389 K achieved at the 20% CuO loading.
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Cites
Generalized syntheses of large-pore mesoporous metal oxides with semicrystalline frameworks
Yang, P., Zhao, D., Margolese, D. I., Chmelka, B. F., & Stucky, G. D. (1998) · Nature · doi:10.1038/24132 · Cited by 2,493
Cited by
Ordered mesoporous metal oxides: synthesis and applications
Ren, Y., Ma, Z., & Bruce, P. G. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35086f · Cited by 768
Porous Metal Oxides as Gas Sensors
Tiemann, M. (2007) · Chemistry – A European Journal · doi:10.1002/chem.200700927 · Cited by 675
On the Synergetic Catalytic Effect in Heterogeneous Nanocomposite Catalysts
Shi, J. (2013) · Chemical Reviews · doi:10.1021/cr3002752 · Cited by 652
Self-citationSynthesis of non-siliceous mesoporous oxides
Gu, D., & Schüth, F. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60155b · Cited by 584
Metadata
- Authors
- Shen, W., Dong, X., Zhu, Y., Chen, H., & Shi, J.
- Venue
- Microporous and Mesoporous Materials
- Publisher
- Elsevier BV
- Published
- 2005-10
- Volume
- 85
- Issue
- 1-2
- Pages
- 157-162
- ISSN
- 1387-1811 (ISSN-L)
- OpenAlex
- W1977193767
- Cited by
- 187
- References
- 1
- FWCI
- 6.05
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shen, W., Dong, X., Zhu, Y., Chen, H., & Shi, J. (2005). Mesoporous CeO2 and CuO-loaded mesoporous CeO2: Synthesis, characterization, and CO catalytic oxidation property. Microporous and Mesoporous Materials. https://doi.org/10.1016/j.micromeso.2005.06.006
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