The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Beyond the top of the volcano? – A unified approach to electrocatalytic oxygen reduction and oxygen evolution
Open accessAbstract
We study the oxygen reduction (ORR) and the oxygen evolution reaction (OER) and based on previous obtained mechanistic insight we provide a unified general analysis of the two reactions simultaneously. The analysis shows that control over at least two independent binding energies is required to obtain a reversible perfect catalyst for both ORR and OER. Often only the reactivity of the surface is changed by changing from one material to another and all binding energies scale with the reactivity. We investigate the limitation in efficiency imposed by these linear scaling relations. This analysis gives rise to a double volcano for ORR and OER, with a region in between, forbidden by the scaling relations. The reversible perfect catalyst for both ORR and OER would fall into this “forbidden region”. Previously, we have found that hydrogen acceptor functionality on oxide surfaces can improve the catalytic performance for OER beyond the limitations originating from the scaling relations. We use this concept to search for promising combinations of binding sites and hydrogen donor/acceptor sites available in transition metal doped graphene, which can act as a catalyst for ORR and OER. We find that MnN4-site embedded in graphene by itself or combined with a COOH is a promising combination for a great combined ORR/OER catalyst.
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Cites
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode
Nørskov, J. K., Rossmeisl, J., Logadottir, A., Lindqvist, L., Kitchin, J. R., Bligaard, T., & Jónsson, H. (2004) · The Journal of Physical Chemistry B · doi:10.1021/jp047349j · Cited by 13,153
Self-citationBenchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
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Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
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Self-citationImproved Oxygen Reduction Activity on Pt 3 Ni(111) via Increased Surface Site Availability
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Computational high-throughput screening of electrocatalytic materials for hydrogen evolution
Greeley, J., Jaramillo, T. F., Bonde, J., Chorkendorff, I., & Nørskov, J. K. (2006) · Nature Materials · doi:10.1038/nmat1752 · Cited by 4,097
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Cited by
Understanding Catalytic Activity Trends in the Oxygen Reduction Reaction
Kulkarni, A., Siahrostami, S., Patel, A., & Nørskov, J. K. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00488 · Cited by 2,742
Self-citationMaterials Design for Rechargeable Metal-Air Batteries
Wang, H.-F., & Xu, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.008 · Cited by 580
Strategies to break linear scaling relationships
Pérez-Ramírez, J., & López, N. (2019) · Nature Catalysis · doi:10.1038/s41929-019-0376-6 · Cited by 528
Recent Progresses in Electrocatalysts for Water Electrolysis
Khan, M. A., Zhao, H., Zou, W., Chen, Z., Cao, W., Fang, J., Xu, J., Zhang, L., & Zhang, J. (2018) · Electrochemical Energy Reviews · doi:10.1007/s41918-018-0014-z · Cited by 527
What Makes High‐Entropy Alloys Exceptional Electrocatalysts?
Löffler, T., Ludwig, A., Rossmeisl, J., & Schuhmann, W. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202109212 · Cited by 464
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Metadata
- Authors
- Busch, M., Halck, N. B., Kramm, U. I., Siahrostami, S., Krtil, P., & Rossmeisl, J.
- Venue
- Nano Energy
- Publisher
- Elsevier BV
- Published
- 2016-11
- Volume
- 29
- Pages
- 126-135
- ISSN
- 2211-2855 (ISSN-L)
- OpenAlex
- W2337261154
- Cited by
- 344
- References
- 8
- FWCI
- 7.42
- Type
- journal article
- Language
- en
- Open access
- green
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