The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Nitrogen-coordinated single Fe sites for efficient electrocatalytic N2 fixation in neutral media
Abstract
Abstract Electrocatalytic nitrogen reduction reaction (NRR) for NH3 generation under ambient conditions presents a promising alternative to the conventional Haber–Bosch process. Here, we report a Fe single-atom catalyst for ambient electrochemical NH3 synthesis. This catalyst achieves high Faradaic efficiency (18.6 ± 0.8%) and NH3 yield rate (62.9 ± 2.7 μg h−1 mgcat.−1) in neutral aqueous electrolyte at room temperature and −0.4 V versus reversible hydrogen electrode. Furthermore, this catalyst exhibits a negligible activity decay during electrolysis for 24 h. X-ray absorption fine structure analyses and theoretical calculations reveal that atomically dispersed single Fe species are stabilized by N in Fe–N4 configuration, which is favorable for N2 activation. This work opens new opportunities for developing advanced single atomic site catalysts for NH3 synthesis via NRR.
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Zhang, L., Han, L., Liu, H., Liu, X., & Luo, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201706921 · Cited by 532
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Cited by
Yang, Y., & Mu, T. (2021) · Green Chemistry · doi:10.1039/d1gc00914a · Cited by 539
Metal‐Nitrogen‐Doped Carbon Materials as Highly Efficient Catalysts: Progress and Rational Design
Shi, Z., Yang, W., Gu, Y., Liao, T., & Sun, Z. (2020) · Advanced Science · doi:10.1002/advs.202001069 · Cited by 470
Recent Advances in MOF‐Derived Single Atom Catalysts for Electrochemical Applications
Song, Z., Zhang, L., Doyle‐Davis, K., Fu, X., Luo, J., & Sun, X. (2020) · Advanced Energy Materials · doi:10.1002/aenm.202001561 · Cited by 412
Self-citationAdvances in iron-based electrocatalysts for nitrate reduction
Yuan, S., Xue, Y., Ma, R., Ma, Q., Chen, Y., & Fan, J. (2023) · Science of The Total Environment · doi:10.1016/j.scitotenv.2023.161444 · Cited by 117
Metadata
- Authors
- Lü, F., Zhao, S., Guo, R., He, J., Peng, X., Bao, H., Fu, J., Han, L., Qi, G., Luo, J., Tang, X., & Liu, X.
- Venue
- Nano Energy
- Publisher
- Elsevier BV
- Published
- 2019-07
- Volume
- 61
- Pages
- 420-427
- ISSN
- 2211-2855 (ISSN-L)
- OpenAlex
- W2942845693
- Cited by
- 424
- References
- 1
- FWCI
- 12.92
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lü, F., Zhao, S., Guo, R., He, J., Peng, X., Bao, H., Fu, J., Han, L., Qi, G., Luo, J., Tang, X., & Liu, X. (2019). Nitrogen-coordinated single Fe sites for efficient electrocatalytic N2 fixation in neutral media. Nano Energy. https://doi.org/10.1016/j.nanoen.2019.04.092
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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