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Pyroelectric effect in CdS nanorods decorated with a molecular Co-catalyst for hydrogen evolution
Open accessAbstract
Abstract Hexagonal cadmium sulfide (CdS) with a noncentro-symmetric structure exhibits piezoelectric and pyroelectric effect due to spontaneous polarization changes companied by temperature variation. However, its pyroelectric effect in pyroelectro-catalytic hydrogen evolution has not been well identified. Herein, we found that CdS nanorods decorated with an organic molecule 2-mercaptobenzimidazole (2MBI) can greatly enhance the pyroelectro-catalytic hydrogen evolution activity. The 2MBI acted as a molecular co-catalyst improves the pyroelectric property of CdS and enhances the separation of pyroelectro-induced charges. Under thermal cycling between 25 °C and 55 °C, CdS-2MBI shows apparently improved pyroelectro-catalytic H2 evolution activity, which is about 5 folds of that for CdS alone. This work may initiate a new prospect for pyroelectric effect in photocatalysis, such as the photocatalytic hydrogen evolution under natural temperature fluctuations.
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Wang, Q., Hisatomi, T., Jia, Q., Tokudome, H., Zhong, M., Wang, C., Pan, Z., Takata, T., Nakabayashi, M., Shibata, N., et al. (2016) · Nature Materials · doi:10.1038/nmat4589 · Cited by 1,684
Cited by
Li, X., Wang, W., Dong, F., Zhang, Z., Han, L., Luo, X., Huang, J., Feng, Z., Chen, Z., Jia, G., et al. (2021) · ACS Catalysis · doi:10.1021/acscatal.0c05354 · Cited by 357
Metadata
- Authors
- Zhang, M., Hu, Q., Ma, K., Ding, Y., & Li, C.
- Venue
- Nano Energy
- Publisher
- Elsevier BV
- Published
- 2020-07
- Volume
- 73
- Pages
- 104810
- ISSN
- 2211-2855 (ISSN-L)
- OpenAlex
- W3017073436
- Cited by
- 200
- References
- 1
- FWCI
- 6.50
- Type
- journal article
- Language
- en
- Open access
- green
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