Cited by 158Advanced oxidation water treatmentEnvironmental remediation with nanomaterialsPesticide and Herbicide Environmental Studies

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Heterogeneous electro–Fenton using three–dimension NZVI–BC electrodes for degradation of neonicotinoid wastewater

Zhang, Chao, Li, Feng, Wen, Rubing, Zhang, Huike, Elumalai, Punniyakotti, Zheng, Qi, Chen, Hongyu, Yang, Yujie, Huang, Mingzhi, Ying, Guangguo·2020·Water Research

DOI 10.1016/j.watres.2020.115975

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Abstract

Neonicotinoids (NEOs), as the most widely used pesticides, pose a serious threat to water ecosystems, especially clothianidin (CLO). However, the degradation behavior of CLO, as a new type of persistent organic pollutant, is rarely studied in wastewater treatment. To bridge this gap, heterogeneous electro-Fenton system using three-dimension electrodes made of biochar-supported zero-valent iron nanoparticle hybrid material (NZVI-BC), abbreviated as 3D-ICE-EF system, is invented and initially applied in CLO wastewater degradation, without the addition of Fenton reagent. NZVI-BC in 3D-ICE-EF system can concentrate CLO on electrodes by excellent adsorption and effectively eliminate it to achieve self-cleaning effect. In addition, the deposition of iron mud (Fe(OH)3) and the circular utilization of Fe in Fenton system is effectively improved by the addition of hydroquinone (HQ) in 3D-ICE-EF system. The pH applicable scope of Fenton system is extended to alkaline condition by the applications of NZVI-BC electrodes. The increase in the acidity of electrolyte is considered the primary reason of the high degradation efficiency of CLO in 3D-ICE-EF system at an initial pH of 9.0. The degradation performance of 3D-ICE-EF system tends to be promoted by the increase of current intensity and air flow rate. Seven plausible mechanisms of CLO degradation were identified in 3D-ICE-EF system. The ecotoxicity evaluation of degradation products indicated that CLO degradation in 3D-ICE-EF system exhibits a remarkable tendency to reduce toxicity levels.

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Authors: Zhang, C., Li, F., Wen, R., Zhang, H., Elumalai, P., Zheng, Q., Chen, H., Yang, Y., Huang, M., & Ying, G.
Affiliations: South China Normal University (CN)
South China University of Technology (CN)
Corresponding author: Li, Feng
Huang, Mingzhi
ORCID: Zhang, Chao
Li, Feng
Zhang, Huike
Elumalai, Punniyakotti
Zheng, Qi
Yang, Yujie
Huang, Mingzhi
Venue: Water Research
Publisher: Elsevier BV
Published: 2020-09
Volume: 182
Pages: 115975
ISSN: 0043-1354 (ISSN-L)
DOI: 10.1016/j.watres.2020.115975
OpenAlex: W3029851150
Cited by: 158
References: 52
Citations by year: 2026: 12 · 2025: 16 · 2024: 31 · 2023: 33 · 2022: 39 · 2021: 26 · 2020: 1
FWCI: 7.70
Type: journal article
Language: en
Open access: closed
Licence: www.elsevier.com/tdm/userlicense/1.0/ (tdm)
www.elsevier.com/legal/tdmrep-license (tdm)
Locations: Water Research (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China
Natural Science Foundation of Guangdong Province
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Advanced oxidation water treatment
Physical Sciences › Environmental Science › Environmental Engineering › Environmental remediation with nanomaterials
Physical Sciences › Environmental Science › Pollution › Pesticide and Herbicide Environmental Studies
Keywords: neonicotinoids, clothianidin, electro-Fenton, heterogeneous electro-Fenton, nanoscale zero-valent iron, three-dimensional electrodes, pesticide wastewater treatment, hydroquinone, iron recycling, alkaline tolerance, degradation mechanism, adsorption
MeSH terms: Neonicotinoids, Electrodes, Hydrogen Peroxide, Water Pollutants, Chemical, Ecosystem, Wastewater

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Heterogeneous electro–Fenton using three–dimension NZVI–BC electrodes for degradation of neonicotinoid wastewater

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