Enzyme-catalyzed polymerization and degradation of copolymers prepared from ϵ-caprolactone and poly(ethylene glycol)
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A series of PCL-PEG and PCL-PEG-PCL block copolymers were successfully synthesized for the first time using lipase CA.
“A series of PCL-PEG and PCL-PEG-PCL block copolymers were successfully synthesized for the first time using lipase CA [168].”
From Recent advances in the synthesis of aliphatic polyesters by ring-opening polymerization☆ (2008) · cites this paper as [168]
Biodegradable copolymers, such as poly(ester-co-carbonate)s, copolycarbonates and polyethylene glycol-polyester block copolymer, have been produced.
“Biodegradable copolymers, such as poly(ester-co-carbonate)s [166], copolycarbonates [167] and polyethylene glycol-polyester block copolymer [168] have been produced.”
From Recent advances in the synthesis of aliphatic polyesters by ring-opening polymerization☆ (2008) · cites this paper as [168]
Lipases were shown to degrade PCL, PLLA, poly(g-butyrolactone), PHB, poly(butylene succinate adipate), PCL/PBS blend and poly(propylene carbonate) in PBS at 37 °C, producing mainly short oligomers.
“Lipases were shown to degrade PCL, [504][505][506][507][508]504,505 PLLA,509 poly(g-butyrolactone), 507 PHB, 508,510 poly(butylene succinate adipate), 511 PCL/PBS blend 511 and poly(propylene carbonate) 508 in PBS at 37 °C, producing mainly short oligomers.”
From Catalysis as an Enabling Science for Sustainable Polymers (2018) · cites this paper as [506]
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References 22 · Cited by 118
- Authors
- He, F., Li, S., Vert, M., & Zhuo, R.
- Affiliations
- Wuhan University (CN)
- Corresponding author
- He, Feng
- Venue
- Polymer
- Publisher
- Elsevier BV
- Published
- 2003-08
- Volume
- 44
- Issue
- 18
- Pages
- 5145-5151
- ISSN
- 0032-3861 (ISSN-L)
- OpenAlex
- W1977409608
- Cited by
- 118
- References
- 22
- Citations by year
- 2026: 1 · 2025: 3 · 2023: 2 · 2022: 2 · 2021: 7 · 2020: 2 · 2019: 3 · 2018: 8 · 2017: 5 · 2016: 4 · 2015: 4 · 2014: 5 · 2013: 6 · 2012: 8
- FWCI
- 2.64
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Polymer (publishedVersion)
- HAL (submittedVersion)
- Topics
- Physical Sciences › Materials Science › Biomaterials › biodegradable polymer synthesis and properties
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Biology › Enzyme Catalysis and Immobilization
- Physical Sciences › Materials Science › Polymers and Plastics › Polymer crystallization and properties
- Keywords
- polycaprolactone, polyethylene glycol, Novozym 435, lipase B, diblock copolymers, triblock copolymers, enzymatic degradation, Pseudomonas lipase, semicrystalline polymers, biodegradable polymers, solvent casting
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