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Structural Evolution from Metal–Organic Framework to Hybrids of Nitrogen-Doped Porous Carbon and Carbon Nanotubes for Enhanced Oxygen Reduction Activity
Abstract
A series of hybrids of nitrogen-doped graphitic porous carbon and carbon nanotubes (NGPC/NCNTs) are readily prepared in a stepwise manner by using a typical metal–organic framework (MOF-5) and urea as the carbon and nitrogen precursors, and nickel as the graphitization catalyst, respectively. These NGPC/NCNTs hybrids have demonstrated prominent catalytic activities toward oxygen reduction reaction (ORR) in alkaline medium. Compared to the benchmark Pt/C catalyst, the optimized NGPC/NCNT-900 (annealed at 900 °C) exhibits superior catalytic activity, durability and methanol tolerance, which makes it one of the best ORR electrocatalysts derived from MOFs. The promising properties in NGPC/NCNT-900 are mainly attributed to synergistic contributions of its unique hybrid structure, rich nitrogen doping, high graphitic degree, and large surface area. This attractive route for the preparation of NGPC/NCNTs holds promise for general use of a great number of available and yet rapidly growing MOFs in constructing high-performance carbon-based ORR electrocatalysts.
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Cites
Design of electrocatalysts for oxygen- and hydrogen-involving energy conversion reactions
Jiao, Y., Zheng, Y., Jaroniec, M., & Qiao, S. Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00470a · Cited by 5,388
Recent advancements in Pt and Pt-free catalysts for oxygen reduction reaction
Nie, Y., Li, L., & Wei, Z. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00484a · Cited by 2,156
Zhong, H., Wang, J., Zhang, Y., Xu, W., Xing, W., Xu, D., Zhang, Y., & Zhang, X. (2014) · Angewandte Chemie International Edition · doi:10.1002/anie.201408990 · Cited by 938
Electrocatalytic H 2 production from seawater over Co, N-codoped nanocarbons
Gao, S., Li, G.-D., Liu, Y., Chen, H., Feng, L.-L., Wang, Y., Yang, M., Wang, D., Wang, S., & Zou, X. (2015) · Nanoscale · doi:10.1039/c4nr04924a · Cited by 180
Cited by
Design Strategies toward Advanced MOF‐Derived Electrocatalysts for Energy‐Conversion Reactions
Liu, J., Zhu, D., Guo, C., Vasileff, A., & Qiao, S. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201700518 · Cited by 668
Metal organic frameworks as precursors for the manufacture of advanced catalytic materials
Oar-Arteta, L., Wezendonk, T., Sun, X., Kapteijn, F., & Gascon, J. (2017) · Materials Chemistry Frontiers · doi:10.1039/c7qm00007c · Cited by 361
Chen, X., Gao, H., Xing, L., Dong, W., Li, A., Cheng, P., Liu, P., & Wang, G. (2019) · Energy Storage Materials · doi:10.1016/j.ensm.2018.08.024 · Cited by 128
Mukhiya, T., Muthurasu, A., Tiwari, A. P., Chhetri, K., Chae, S.-H., Kim, H., Dahal, B., Lee, B. M., & Kim, H. Y. (2021) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.1c04104 · Cited by 67
Metadata
- Authors
- Zhang, L., Wang, X., Wang, R., & Hong, M.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-11-10
- Volume
- 27
- Issue
- 22
- Pages
- 7610-7618
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2271277358
- Cited by
- 238
- References
- 4
- FWCI
- 7.72
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, L., Wang, X., Wang, R., & Hong, M. (2015). Structural Evolution from Metal–Organic Framework to Hybrids of Nitrogen-Doped Porous Carbon and Carbon Nanotubes for Enhanced Oxygen Reduction Activity. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.5b02708
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