The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Poly(ethyl α-cyanoacrylate)-Based Artificial Solid Electrolyte Interphase Layer for Enhanced Interface Stability of Li Metal Anodes
Abstract
The inhomogeneous deposition/dissolution of Li metal and an unstable SEI layer are still tough issues for lithium metal batteries, causing severe safety problems and low Coulombic efficiency. In this paper, we design an artificial SEI layer based on in situ polymerization of ethyl α-cyanoacrylate precursor with LiNO 3 additive. The CN– and NO 3 – groups can react with lithium metal during cycling to form a nitrogenous interface inorganic layer, facilitating ions conduction and blocking further undesirable interface reaction. The poly(ethyl α-cyanoacrylate) with excellent mechanical property presents as the dominate organic species in the artificial SEI layer to offer a uniform and firm protective outer layer. A lithium metal battery with this artificial SEI film exhibits a capacity retention of 93% even after 500 cycles at a rate of 2C. A smooth surface morphology of the lithium metal anode is obtained without any cracks and dendrites.
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Citations
Cites
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Artificial Interphases for Highly Stable Lithium Metal Anode
Xu, R., Cheng, X.-B., Yan, C., Zhang, X.-Q., Xiao, Y., Zhao, C.-Z., Huang, J.-Q., & Zhang, Q. (2019) · Matter · doi:10.1016/j.matt.2019.05.016 · Cited by 721
Lithium metal anodes: Present and future
Wang, R., Cui, W., Chu, F., & Wu, F. (2020) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2019.12.024 · Cited by 544
In situ polymerization process: an essential design tool for lithium polymer batteries
Vijayakumar, V., Anothumakkool, B., Kurungot, S., Winter, M., & Nair, J. R. (2021) · Energy & Environmental Science · doi:10.1039/d0ee03527k · Cited by 365
Polymers in Lithium‐Ion and Lithium Metal Batteries
Li, J., Cai, Y., Wu, H., Yu, Z., Yan, X., Zhang, Q., Gao, T. Z., Liu, K., Jia, X., & Bao, Z. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202003239 · Cited by 348
Perspectives for restraining harsh lithium dendrite growth: Towards robust lithium metal anodes
Wu, F., Yuan, Y.-X., Cheng, X.-B., Bai, Y., Li, Y., Wu, C., & Zhang, Q. (2018) · Energy Storage Materials · doi:10.1016/j.ensm.2018.03.024 · Cited by 319
Metadata
- Authors
- Hu, Z., Zhang, S., Dong, S., Li, W., Li, H., Cui, G., & Chen, L.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-05-22
- Volume
- 29
- Issue
- 11
- Pages
- 4682-4689
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2615953586
- Cited by
- 221
- References
- 1
- FWCI
- 11.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, Z., Zhang, S., Dong, S., Li, W., Li, H., Cui, G., & Chen, L. (2017). Poly(ethyl α-cyanoacrylate)-Based Artificial Solid Electrolyte Interphase Layer for Enhanced Interface Stability of Li Metal Anodes. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.7b00091
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