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Pd NPs-Loaded Homochiral Covalent Organic Framework for Heterogeneous Asymmetric Catalysis
Abstract
We herein report the fabrication of a palladium nanoparticles (Pd NPs) loaded homochiral covalent organic framework using S -(+)-2-methylpiperazine and cyanuric chloride (Pd@CCOF-MPC) ( 2 ) via a very facile chemical approach. The chiral COF support of 1 (CCOF-MPC) is synthesized by the combination of cyanuric chloride and S -(+)-2-methylpiperazine at 90 °C for 36 h, and the Pd NPs-loaded Pd@CCOF-MPC ( 2 ) is prepared via sequential solution impregnation and NaBH 4 reduction at room temperature. 2, as a highly active reusable asymmetric heterogeneous composite catalyst, is able to effectively promote the Henry reaction and reductive Heck reaction in high yield with excellent stereoselectivity.
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Scheuermann, G. M., Rumi, L., Steurer, P., Bannwarth, W., & Mülhaupt, R. (2009) · Journal of the American Chemical Society · doi:10.1021/ja901105a · Cited by 1,163
Cited by
Liu, R., Tan, K. T., Gong, Y., Chen, Y., Li, Z., Xie, S., He, T., Lu, Z., Yang, H., & Jiang, D. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00620c · Cited by 1,083
Chiral covalent organic frameworks: design, synthesis and property
Han, X., Yuan, C., Hou, B., Liu, L., Li, H., Liu, Y., & Cui, Y. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00009d · Cited by 478
Metadata
- Authors
- Ma, H.-C., Kan, J.-L., Chen, G.-J., Chen, C.-X., & Dong, Y.-B.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-17
- Volume
- 29
- Issue
- 15
- Pages
- 6518-6524
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2729048283
- Cited by
- 171
- References
- 1
- FWCI
- 8.36
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ma, H.-C., Kan, J.-L., Chen, G.-J., Chen, C.-X., & Dong, Y.-B. (2017). Pd NPs-Loaded Homochiral Covalent Organic Framework for Heterogeneous Asymmetric Catalysis. Chemistry of Materials. https://doi.org/10.1021/acs.chemmater.7b02131
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