The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Highly Efficient Performance and Conversion Pathway of Photocatalytic NO Oxidation on SrO-Clusters@Amorphous Carbon Nitride
Open accessAbstract
This work demonstrates the first molecular-level conversion pathway of NO oxidation over a novel SrO-clusters@amorphous carbon nitride (SCO-ACN) photocatalyst, which is synthesized via copyrolysis of urea and SrCO 3 . The inclusion of SrCO 3 is crucial in the formation of the amorphous carbon nitride (ACN) and SrO clusters by attacking the intralayer hydrogen bonds at the edge sites of graphitic carbon nitride (CN). The amorphous nature of ACN can promote the transportation, migration, and transformation of charge carriers on SCO-ACN. And the SrO clusters are identified as the newly formed active centers to facilitate the activation of NO via the formation of Sr-NO δ(+), which essentially promotes the conversion of NO to the final products. The combined effects of the amorphous structure and SrO clusters impart outstanding photocatalytic NO removal efficiency to the SCO-ACN under visible-light irradiation. To reveal the photocatalytic mechanism, the adsorption and photocatalytic oxidation of NO over CN and SCO-ACN are analyzed by in situ DRIFTS, and the intermediates and conversion pathways are elucidated and compared. This work presents a novel in situ DRIFTS-based strategy to explore the photocatalytic reaction pathway of NO oxidation, which is quite beneficial to understand the mechanism underlying the photocatalytic reaction and advance the development of photocatalytic technology for environmental remediation.
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Cites
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Selective Breaking of Hydrogen Bonds of Layered Carbon Nitride for Visible Light Photocatalysis
Kang, Y., Yang, Y., Yin, L., Kang, X., Wang, L., Liu, G., & Cheng, H. (2016) · Advanced Materials · doi:10.1002/adma.201601567 · Cited by 626
West, J. J., Cohen, A., Dentener, F., Brunekreef, B., Zhu, T., Armstrong, B., Bell, M. L., Brauer, M., Carmichael, G., Costa, D. L., et al. (2016) · Environmental Science & Technology · doi:10.1021/acs.est.5b03827 · Cited by 390
Cited by
Mousavi, M., Habibi-Yangjeh, A., & Pouran, S. R. (2018) · Journal of Materials Science: Materials in Electronics · doi:10.1007/s10854-017-8166-x · Cited by 560
Hasija, V., Raizada, P., Sudhaik, A., Sharma, K., Kumar, A., Singh, P., Jonnalagadda, S. B., & Thakur, V. K. (2019) · Applied Materials Today · doi:10.1016/j.apmt.2019.04.003 · Cited by 503
Roles of N-Vacancies over Porous g-C3N4 Microtubes during Photocatalytic NOx Removal
Wang, Z., Huang, Y., Chen, M., Shi, X., Zhang, Y., Cao, J., Ho, W., & Lee, S. C. (2019) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.8b21987 · Cited by 287
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Metadata
- Authors
- Cui, W., Li, J., Dong, F., Sun, Y., Jiang, G., Cen, W., Lee, S. C., & Wu, Z.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-08-30
- Volume
- 51
- Issue
- 18
- Pages
- 10682-10690
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2748715882
- Cited by
- 248
- References
- 3
- FWCI
- 8.25
- Type
- journal article
- Language
- en
- Open access
- green
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- Cui, W., Li, J., Dong, F., Sun, Y., Jiang, G., Cen, W., Lee, S. C., & Wu, Z. (2017). Highly Efficient Performance and Conversion Pathway of Photocatalytic NO Oxidation on SrO-Clusters@Amorphous Carbon Nitride. Environmental Science & Technology. https://doi.org/10.1021/acs.est.7b00974
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