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Acridinium-Based Photocatalysts: A Sustainable Option in Photoredox Catalysis
Abstract
The emergence of visible light photoredox catalysis has enabled the productive use of lower energy radiation, leading to highly selective reaction platforms. Polypyridyl complexes of iridium and ruthenium have served as popular photocatalysts in recent years due to their long excited state lifetimes and useful redox windows, leading to the development of diverse photoredox-catalyzed transformations. The low abundances of Ir and Ru in the earth's crust and, hence, cost make these catalysts nonsustainable and have limited their application in industrial-scale manufacturing. Herein, we report a series of novel acridinium salts as alternatives to iridium photoredox catalysts and show their comparability to the ubiquitous [Ir(dF-CF3-ppy)2(dtbpy)](PF6).
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Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
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Barham, J. P., & König, B. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201913767 · Cited by 448
Pearson, R. M., Lim, C.-H., McCarthy, B. G., Musgrave, C. B., & Miyake, G. M. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b08068 · Cited by 339
Wu, C., Corrigan, N., Lim, C.-H., Liu, W., Miyake, G., & Boyer, C. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00409 · Cited by 259
Metadata
- Authors
- Joshi-Pangu, A., Lévesque, F., Roth, H. G., Oliver, S. F., Campeau, L.-C., Nicewicz, D., & DiRocco, D. A.
- Venue
- The Journal of Organic Chemistry
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-07-25
- Volume
- 81
- Issue
- 16
- Pages
- 7244-7249
- ISSN
- 0022-3263 (ISSN-L)
- 1520-6904
- OpenAlex
- W2480067148
- Cited by
- 410
- References
- 1
- FWCI
- 12.77
- Type
- journal article
- Language
- en
- Open access
- closed
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- Joshi-Pangu, A., Lévesque, F., Roth, H. G., Oliver, S. F., Campeau, L.-C., Nicewicz, D., & DiRocco, D. A. (2016). Acridinium-Based Photocatalysts: A Sustainable Option in Photoredox Catalysis. The Journal of Organic Chemistry. https://doi.org/10.1021/acs.joc.6b01240
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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