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X-ray Photoelectron Spectroscopic Investigation of Plasma-Enhanced Chemical Vapor Deposited NiOx, NiOx(OH)y, and CoNiOx(OH)y: Influence of the Chemical Composition on the Catalytic Activity for the Oxygen Evolution Reaction
Open accessAbstract
Abstract We report here the plasma-enhanced chemical vapor deposition and electrocatalytic characterization of pure NiOx and NiOx(OH)y. Whereas NiOx is deposited if oxygen is used as a reactive gas, the use of air as a reactive gas leads to the deposition of the NiOx(OH)y, which is electrochemically more active than the NiOx. By recording X-ray photoelectron spectra from the as-deposited catalysts and after their electrochemical investigations, we determined that the electrochemical activity correlates with the amount of hydroxide sites on the surface. Such a behavior was already observed for CoOx and CoOx(OH)y. As a consequence, CoNiOx(OH)y was deposited using air as a reactive gas to study the influence of nickel on the electronic structure of CoOx(OH)y and its effect on the electrochemical activity.
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Citations
Cites
Benchmarking Heterogeneous Electrocatalysts for the Oxygen Evolution Reaction
McCrory, C. C. L., Jung, S., Peters, J. C., & Jaramillo, T. F. (2013) · Journal of the American Chemical Society · doi:10.1021/ja407115p · Cited by 7,026
Cited by
Boyd, C. C., Shallcross, R. C., Moot, T., Kerner, R., Bertoluzzi, L., Onno, A., Kavadiya, S., Chosy, C., Wolf, E. J., Werner, J., et al. (2020) · Joule · doi:10.1016/j.joule.2020.06.004 · Cited by 639
Catalyst Preparation with Plasmas: How Does It Work?
Wang, Z., Zhang, Y., Neyts, E. C., Cao, X., Zhang, X., Jang, B. W.-L., & Liu, C.-J. (2018) · ACS Catalysis · doi:10.1021/acscatal.7b03723 · Cited by 494
Zhao, G., Li, P., Cheng, N., Dou, S. X., & Sun, W. (2020) · Advanced Materials · doi:10.1002/adma.202000872 · Cited by 333
Anion Exchange Membrane Water Electrolysis Based on Nickel Ferrite Catalysts
Caprì, A., Gatto, I., Lo Vecchio, C., Trocino, S., Carbone, A., & Baglio, V. (2023) · ChemElectroChem · doi:10.1002/celc.202201056 · Cited by 57
Metadata
- Authors
- Weidler, N., Schuch, J., Knaus, F., Stenner, P., Hoch, S., Maljusch, A., Schäfer, R., Kaiser, B., & Jaegermann, W.
- Venue
- The Journal of Physical Chemistry C
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-03-19
- Volume
- 121
- Issue
- 12
- Pages
- 6455-6463
- ISSN
- 1932-7447 (ISSN-L)
- 1932-7455
- OpenAlex
- W2591299087
- Cited by
- 297
- References
- 1
- FWCI
- 5.05
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- CoChat. (2026). Citation check: X-ray Photoelectron Spectroscopic Investigation of Plasma-Enhanced Chemical Vapor Deposited NiOx, NiOx(OH)y, and CoNiOx(OH)y: Influence of the Chemical Composition on the Catalytic Activity for the Oxygen Evolution Reaction. https://app.cochat.ai/papers/10.1021/acs.jpcc.6b12652
- The paper
- Weidler, N., Schuch, J., Knaus, F., Stenner, P., Hoch, S., Maljusch, A., Schäfer, R., Kaiser, B., & Jaegermann, W. (2017). X-ray Photoelectron Spectroscopic Investigation of Plasma-Enhanced Chemical Vapor Deposited NiOx, NiOx(OH)y, and CoNiOx(OH)y: Influence of the Chemical Composition on the Catalytic Activity for the Oxygen Evolution Reaction. The Journal of Physical Chemistry C. https://doi.org/10.1021/acs.jpcc.6b12652
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