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Organometal Trihalide Perovskite Single Crystals: A Next Wave of Materials for 25% Efficiency Photovoltaics and Applications Beyond?
Abstract
Hybrid perovskite single crystals have been recently revealed to have superior optoelectronic properties to perovskite polycrystalline thin films, especially the extraordinarily long carrier diffusion length due to the eliminated grain boundaries. One question that naturally arises is whether the single crystal hybrid perovskites can be a next wave of photoactive materials for even higher-efficiency devices. This Perspective presents an overview of the historic evolution in understanding of carrier diffusion length in CH 3 NH 3 PbI 3, the initial investigations of the synthesis of single crystalline hybrid perovskites, and the characterization of their optoelectronic properties. Our analysis indicates that single crystalline perovskite materials have potential to further boost photovoltaic device power conversion efficiency to 25%. The potential opportunities for the fundamental study of the perovskite intrinsic properties, particularly the carrier mobility and carrier recombination lifetime, and other fields such as radiation detectors are also briefed.
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Stranks, S. D., Eperon, G. E., Grancini, G., Menelaou, C., Alcocer, M. J. P., Leijtens, T., Herz, L. M., Petrozza, A., & Snaith, H. J. (2013) · Science · doi:10.1126/science.1243982 · Cited by 10,413
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors
Zhu, H., Fu, Y., Meng, F., Wu, X., Gong, Z., Ding, Q., Gustafsson, M. V., Trinh, M. T., Jin, S., & Zhu, X.-Y. (2015) · Nature Materials · doi:10.1038/nmat4271 · Cited by 2,836
Impact of microstructure on local carrier lifetime in perovskite solar cells
de Quilettes, D. W., Vorpahl, S. M., Stranks, S. D., Nagaoka, H., Eperon, G. E., Ziffer, M. E., Snaith, H. J., & Ginger, D. S. (2015) · Science · doi:10.1126/science.aaa5333 · Cited by 2,198
Lead iodide perovskite light-emitting field-effect transistor
Chin, X. Y., Cortecchia, D., Yin, J., Bruno, A., & Soci, C. (2015) · Nature Communications · doi:10.1038/ncomms8383 · Cited by 767
Cited by
Brenner, T. M., Egger, D. A., Kronik, L., Hodes, G., & Cahen, D. (2016) · Nature Reviews Materials · doi:10.1038/natrevmats.2015.7 · Cited by 1,557
Printable organometallic perovskite enables large-area, low-dose X-ray imaging
Kim, Y. C., Kim, K. H., Son, D.-Y., Jeong, D.-N., Seo, J.-Y., Choi, Y. S., Han, I. T., Lee, S. Y., & Park, N.-G. (2017) · Nature · doi:10.1038/nature24032 · Cited by 1,206
Ahmadi, M., Wu, T., & Hu, B. (2017) · Advanced Materials · doi:10.1002/adma.201605242 · Cited by 820
Lin, Y., Shen, L., Dai, J., Deng, Y., Wu, Y., Bai, Y., Zheng, X., Wang, J., Fang, Y., Wei, H., et al. (2017) · Advanced Materials · doi:10.1002/adma.201604545 · Cited by 640
Self-citationSynthetic Approaches for Halide Perovskite Thin Films
Dunlap-Shohl, W. A., Zhou, Y., Padture, N. P., & Mitzi, D. B. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00318 · Cited by 631
Metadata
- Authors
- Huang, J., Shao, Y., & Dong, Q.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-08-07
- Volume
- 6
- Issue
- 16
- Pages
- 3218-3227
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2224609287
- Cited by
- 245
- References
- 4
- FWCI
- 17.00
- Type
- journal article
- Language
- en
- Open access
- closed
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- Huang, J., Shao, Y., & Dong, Q. (2015). Organometal Trihalide Perovskite Single Crystals: A Next Wave of Materials for 25% Efficiency Photovoltaics and Applications Beyond? The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.5b01419
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