The DOI matches its Crossref record; 1 of the 1 references it cites were found in a registry or an index.
Role of the Electron Spin Polarization in Water Splitting
Open accessAbstract
We show that in an electrochemical cell, in which the photoanode is coated with chiral molecules, the overpotential required for hydrogen production drops remarkably, as compared with cells containing achiral molecules. The hydrogen evolution efficiency is studied comparing seven different organic molecules, three chiral and four achiral. We propose that the spin specificity of electrons transferred through chiral molecules is the origin of a more efficient oxidation process in which oxygen is formed in its triplet ground state. The new observations are consistent with recent theoretical works pointing to the importance of spin alignment in the water-splitting process.
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Cites
Comparing Photosynthetic and Photovoltaic Efficiencies and Recognizing the Potential for Improvement
Blankenship, R. E., Tiede, D. M., Barber, J., Brudvig, G. W., Fleming, G., Ghirardi, M., Gunner, M. R., Junge, W., Kramer, D. M., Melis, A., et al. (2011) · Science · doi:10.1126/science.1200165 · Cited by 1,638
Cited by
Chiral molecules and the electron spin
Naaman, R., Paltiel, Y., & Waldeck, D. H. (2019) · Nature Reviews Chemistry · doi:10.1038/s41570-019-0087-1 · Cited by 934
Self-citationManipulating spin polarization of titanium dioxide for efficient photocatalysis
Pan, L., Ai, M., Huang, C., Yin, L., Liu, X., Zhang, R., Wang, S., Jiang, Z., Zhang, X., Zou, J.-J., et al. (2020) · Nature Communications · doi:10.1038/s41467-020-14333-w · Cited by 543
Spin-dependent charge transport through 2D chiral hybrid lead-iodide perovskites
Lu, H., Wang, J., Xiao, C., Pan, X., Chen, X., Brunecky, R., Berry, J. J., Zhu, K., Beard, M. C., & Vardeny, Z. V. (2019) · Science Advances · doi:10.1126/sciadv.aay0571 · Cited by 533
Theory of Chirality Induced Spin Selectivity: Progress and Challenges
Evers, F., Aharony, A., Bar‐Gill, N., Entin‐Wohlman, O., Hedegård, P., Hod, O., Jelinek, P., Kamieniarz, G., Lemeshko, M., Michaeli, K., et al. (2022) · Advanced Materials · doi:10.1002/adma.202106629 · Cited by 359
Self-citationMichaeli, K., Kantor-Uriel, N., Naaman, R., & Waldeck, D. H. (2016) · Chemical Society Reviews · doi:10.1039/c6cs00369a · Cited by 291
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Metadata
- Authors
- Mtangi, W., Kiran, V., Fontanesi, C., & Naaman, R.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-12-01
- Volume
- 6
- Issue
- 24
- Pages
- 4916-4922
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2224106144
- Cited by
- 250
- References
- 1
- FWCI
- 2.35
- Type
- journal article
- Language
- en
- Open access
- hybrid
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
