The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Phosphate Ion Functionalization of Perovskite Surfaces for Enhanced Oxygen Evolution Reaction
Abstract
Recent findings revealed that surface oxygen can participate in the oxygen evolution reaction (OER) for the most active catalysts, which eventually triggers a new mechanism for which the deprotonation of surface intermediates limits the OER activity. We propose in this work a “dual strategy” in which tuning the electronic properties of the oxide, such as La 1– x Sr x CoO 3−δ, can be dissociated from the use of surface functionalization with phosphate ion groups (P i ) that enhances the interfacial proton transfer. Results show that the P i functionalized La 0.5 Sr 0.5 CoO 3−δ gives rise to a significant enhancement of the OER activity when compared to La 0.5 Sr 0.5 CoO 3−δ and LaCoO 3 . We further demonstrate that the P i surface functionalization selectivity enhances the activity when the OER kinetics is limited by the proton transfer. Finally, this work suggests that tuning the catalytic activity by such a “dual approach” may be a new and largely unexplored avenue for the design of novel high-performance catalysts.
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Cites
Universality in Oxygen Evolution Electrocatalysis on Oxide Surfaces
Man, I. C., Su, H., Calle‐Vallejo, F., Hansen, H. A., Martínez, J. I., Inoglu, N. G., Kitchin, J., Jaramillo, T. F., Nørskov, J. K., & Rossmeisl, J. (2011) · ChemCatChem · doi:10.1002/cctc.201000397 · Cited by 4,769
Shinagawa, T., Garcia-Esparza, A. T., & Takanabe, K. (2015) · Scientific Reports · doi:10.1038/srep13801 · Cited by 3,287
Toward the rational design of non-precious transition metal oxides for oxygen electrocatalysis
Hong, W. T., Risch, M., Stoerzinger, K. A., Grimaud, A., Suntivich, J., & Shao-Horn, Y. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03869j · Cited by 2,089
Self-citationThe Mechanism of Water Oxidation: From Electrolysis via Homogeneous to Biological Catalysis
Dau, H., Limberg, C., Reier, T., Risch, M., Roggan, S., & Strasser, P. (2010) · ChemCatChem · doi:10.1002/cctc.201000126 · Cited by 1,783
Cited by
A review on fundamentals for designing oxygen evolution electrocatalysts
Song, J., Wei, C., Huang, Z.-F., Liu, C., Zeng, L., Wang, X., & Xu, Z. J. (2020) · Chemical Society Reviews · doi:10.1039/c9cs00607a · Cited by 2,936
Xiao, Z., Huang, Y.-C., Dong, C.-L., Xie, C., Liu, Z., Du, S., Chen, W., Yan, D., Tao, L., Shu, Z., et al. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c00257 · Cited by 1,445
Preferential Cation Vacancies in Perovskite Hydroxide for the Oxygen Evolution Reaction
Chen, D., Qiao, M., Lu, Y., Hao, L., Liu, D., Dong, C., Li, Y., & Wang, S. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201805520 · Cited by 409
He, Z., Hwang, J., Gong, Z., Zhou, M., Zhang, N., Kang, X., Han, J. W., & Chen, Y. (2022) · Nature Communications · doi:10.1038/s41467-022-31484-0 · Cited by 291
Li, C.-F., Shuai, T.-Y., Zheng, L.-R., Tang, H.-B., Zhao, J.-W., & Li, G.-R. (2023) · Chemical Engineering Journal · doi:10.1016/j.cej.2022.138618 · Cited by 149
Metadata
- Authors
- Yang, C., Laberty-Robert, C., Batuk, D., Cibin, G., Chadwick, A. V., Pimenta, V., Yin, W., Zhang, L., Tarascon, J.-M., & Grimaud, A.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2017-07-13
- Volume
- 8
- Issue
- 15
- Pages
- 3466-3472
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2726908471
- Cited by
- 171
- References
- 4
- FWCI
- 3.27
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, C., Laberty-Robert, C., Batuk, D., Cibin, G., Chadwick, A. V., Pimenta, V., Yin, W., Zhang, L., Tarascon, J.-M., & Grimaud, A. (2017). Phosphate Ion Functionalization of Perovskite Surfaces for Enhanced Oxygen Evolution Reaction. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.7b01504
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