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Theory of the Double Layer in Water-in-Salt Electrolytes
Abstract
One challenge in developing the next generation of lithium-ion batteries is the replacement of organic electrolytes, which are flammable and most often contain toxic and thermally unstable lithium salts, with safer, environmentally friendly alternatives. Recently developed water-in-salt electrolytes (WiSEs), which are nonflammable, nontoxic, and also have enhanced electrochemical stability, are promising alternatives. In this work, we develop a simple modified Poisson-Fermi theory for WiSEs, which demonstrates the fine interplay between electrosorption, solvation, and ion correlations. The phenomenological parameters are extracted from molecular dynamics simulations, also performed here. The theory reproduces the WiSEs' electrical double-layer structure with remarkable accuracy.
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Cites
“Water-in-salt” electrolyte enables high-voltage aqueous lithium-ion chemistries
Suo, L., Borodin, O., Gao, T., Olguin, M., Ho, J., Fan, X., Luo, C., Wang, C., & Xu, K. (2015) · Science · doi:10.1126/science.aab1595 · Cited by 3,821
Influence of chloride, water, and organic solvents on the physical properties of ionic liquids
Seddon, K. R., Stark, A., & Torres, M.-J. (2000) · Pure and Applied Chemistry · doi:10.1351/pac200072122275 · Cited by 2,293
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Electrochemical energy storage devices working in extreme conditions
Chen, M., Zhang, Y., Xing, G., Chou, S.-L., & Tang, Y. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00271f · Cited by 346
The Many Deaths of Supercapacitors: Degradation, Aging, and Performance Fading
Pameté, E., Köps, L., Kreth, F. A., Pohlmann, S., Varzi, A., Brousse, T., Balducci, A., & Presser, V. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202301008 · Cited by 328
Electrotunable friction with ionic liquid lubricants
Bresme, F., Kornyshev, A. A., Perkin, S., & Urbakh, M. (2022) · Nature Materials · doi:10.1038/s41563-022-01273-7 · Cited by 105
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Metadata
- Authors
- McEldrew, M., Goodwin, Z. A. H., Kornyshev, A. A., & Bazant, M. Z.
- Venue
- The Journal of Physical Chemistry Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2018-09-19
- Volume
- 9
- Issue
- 19
- Pages
- 5840-5846
- ISSN
- 1948-7185 (ISSN-L)
- OpenAlex
- W2886453734
- Cited by
- 202
- References
- 2
- FWCI
- 15.87
- Type
- journal article
- Language
- en
- Open access
- closed
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- McEldrew, M., Goodwin, Z. A. H., Kornyshev, A. A., & Bazant, M. Z. (2018). Theory of the Double Layer in Water-in-Salt Electrolytes. The Journal of Physical Chemistry Letters. https://doi.org/10.1021/acs.jpclett.8b02543
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