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Synergetic Effects of Inorganic Components in Solid Electrolyte Interphase on High Cycle Efficiency of Lithium Ion Batteries
Abstract
The solid electrolyte interphase (SEI), a passivation layer formed on electrodes, is critical to battery performance and durability. The inorganic components in SEI, including lithium carbonate (Li2CO3) and lithium fluoride (LiF), provide both mechanical and chemical protection, meanwhile control lithium ion transport. Although both Li2CO3 and LiF have relatively low ionic conductivity, we found, surprisingly, that the contact between Li2CO3 and LiF can promote space charge accumulation along their interfaces, which generates a higher ionic carrier concentration and significantly improves lithium ion transport and reduces electron leakage. The synergetic effect of the two inorganic components leads to high current efficiency and long cycle stability.
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Citations
Cites
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Cited by
Review on modeling of the anode solid electrolyte interphase (SEI) for lithium-ion batteries
Wang, A., Kadam, S., Li, H., Shi, S., & Qi, Y. (2018) · npj Computational Materials · doi:10.1038/s41524-018-0064-0 · Cited by 1,639
Self-citationNon-flammable electrolyte enables Li-metal batteries with aggressive cathode chemistries
Fan, X., Chen, L., Borodin, O., Ji, X., Chen, J., Hou, S., Deng, T., Zheng, J., Yang, C., Liou, S.-C., et al. (2018) · Nature Nanotechnology · doi:10.1038/s41565-018-0183-2 · Cited by 1,371
A Growing Appreciation for the Role of LiF in the Solid Electrolyte Interphase
Tan, J., Matz, J., Dong, P., Shen, J., & Ye, M. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202100046 · Cited by 1,019
High-voltage liquid electrolytes for Li batteries: progress and perspectives
Fan, X., & Wang, C. (2021) · Chemical Society Reviews · doi:10.1039/d1cs00450f · Cited by 980
Highly Fluorinated Interphases Enable High-Voltage Li-Metal Batteries
Fan, X., Chen, L., Ji, X., Deng, T., Hou, S., Chen, J., Zheng, J., Wang, F., Jiang, J., Xu, K., et al. (2018) · Chem · doi:10.1016/j.chempr.2017.10.017 · Cited by 961
Metadata
- Authors
- Zhang, Q., Pan, J., Lu, P., Liu, Z., Verbrugge, M. W., Sheldon, B. W., Cheng, Y.-T., Qi, Y., & Xiao, X.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-02-24
- Volume
- 16
- Issue
- 3
- Pages
- 2011-2016
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2279436792
- Cited by
- 472
- References
- 1
- FWCI
- 15.25
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Zhang, Q., Pan, J., Lu, P., Liu, Z., Verbrugge, M. W., Sheldon, B. W., Cheng, Y.-T., Qi, Y., & Xiao, X. (2016). Synergetic Effects of Inorganic Components in Solid Electrolyte Interphase on High Cycle Efficiency of Lithium Ion Batteries. Nano Letters. https://doi.org/10.1021/acs.nanolett.5b05283
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