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Entropic Ligands for Nanocrystals: From Unexpected Solution Properties to Outstanding Processability
Abstract
Solution processability of nanocrystals coated with a stable monolayer of organic ligands (nanocrystal-ligands complexes) is the starting point for their applications, which is commonly measured by their solubility in media. A model described in the other report (10.1021/acs.nanolett.6b00737) reveals that instead of offering steric barrier between inorganic cores, it is the rotation/bending entropy of the C-C σ bonds within typical organic ligands that exponentially enhances solubility of the complexes in solution. Dramatic ligand chain-length effects on the solubility of CdSe-n-alkanoates complexes shall further reveal the power of the model. Subsequently, "entropic ligands" are introduced to maximize the intramolecular entropic effects, which increases solubility of various nanocrystals by 10(2)-10(6). Entropic ligands can further offer means to greatly improve performance of nanocrystals-based electronic and optoelectronic devices.
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Cites
Colloidal nanocrystal synthesis and the organic–inorganic interface
Yin, Y., & Alivisatos, A. P. (2005) · Nature · doi:10.1038/nature04165 · Cited by 3,273
Cited by
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Phan, H. T., & Haes, A. J. (2019) · The Journal of Physical Chemistry C · doi:10.1021/acs.jpcc.9b00913 · Cited by 473
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Kagan, C. R., Bassett, L. C., Murray, C. B., & Thompson, S. M. (2021) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00831 · Cited by 331
Colloidal Halide Perovskite Nanoplatelets: An Exciting New Class of Semiconductor Nanomaterials
Weidman, M. C., Goodman, A. J., & Tisdale, W. A. (2017) · Chemistry of Materials · doi:10.1021/acs.chemmater.7b01384 · Cited by 285
Metadata
- Authors
- Yang, Y., Qin, H., Jiang, M., Lin, L., Fu, T., Dai, X., Zhang, Z., Niu, Y., Cao, H., Jin, Y., Zhao, F., & Peng, X.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-08
- Volume
- 16
- Issue
- 4
- Pages
- 2133-2138
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2285460824
- Cited by
- 245
- References
- 1
- FWCI
- 10.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, Y., Qin, H., Jiang, M., Lin, L., Fu, T., Dai, X., Zhang, Z., Niu, Y., Cao, H., Jin, Y., Zhao, F., & Peng, X. (2016). Entropic Ligands for Nanocrystals: From Unexpected Solution Properties to Outstanding Processability. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b00730
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