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Monolayer Single-Crystal 1T′-MoTe2 Grown by Chemical Vapor Deposition Exhibits Weak Antilocalization Effect
Open accessAbstract
Growth of transition metal dichalcogenide (TMD) monolayers is of interest due to their unique electrical and optical properties. Films in the 2H and 1T phases have been widely studied but monolayers of some 1T'-TMDs are predicted to be large-gap quantum spin Hall insulators, suitable for innovative transistor structures that can be switched via a topological phase transition rather than conventional carrier depletion [ Qian et al. Science 2014 , 346 , 1344 - 1347 ]. Here we detail a reproducible method for chemical vapor deposition of monolayer, single-crystal flakes of 1T'-MoTe2. Atomic force microscopy, Raman spectroscopy, X-ray photoelectron spectroscopy, and transmission electron microscopy confirm the composition and structure of MoTe2 flakes. Variable temperature magnetotransport shows weak antilocalization at low temperatures, an effect seen in topological insulators and evidence of strong spin-orbit coupling. Our approach provides a pathway to systematic investigation of monolayer, single-crystal 1T'-MoTe2 and implementation in next-generation nanoelectronic devices.
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Cites
The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Z 2 Topological Order and the Quantum Spin Hall Effect
Kane, C. L., & Mele, E. J. (2005) · Physical Review Letters · doi:10.1103/physrevlett.95.146802 · Cited by 6,460
Topological Insulators in Three Dimensions
Fu, L., Kane, C. L., & Mele, E. J. (2007) · Physical Review Letters · doi:10.1103/physrevlett.98.106803 · Cited by 4,651
Quantum spin Hall effect in two-dimensional transition metal dichalcogenides
Qian, X., Liu, J., Fu, L., & Li, J. (2014) · Science · doi:10.1126/science.1256815 · Cited by 2,053
Two-dimensional transition metal dichalcogenide nanosheet-based composites
Tan, C., & Zhang, H. (2015) · Chemical Society Reviews · doi:10.1039/c4cs00182f · Cited by 1,605
Cited by
Interface-Assisted Synthesis of 2D Materials: Trend and Challenges
Dong, R., Zhang, T., & Feng, X. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00056 · Cited by 710
Li, H., Li, Y., Aljarb, A., Shi, Y., & Li, L.-J. (2018) · Chemical Reviews · doi:10.1021/acs.chemrev.7b00212 · Cited by 382
Sim, Y., Chae, Y., & Kwon, S.-Y. (2022) · iScience · doi:10.1016/j.isci.2022.105098 · Cited by 47
Metadata
- Authors
- Naylor, C. H., Parkin, W. M., Ping, J., Gao, Z., Zhou, Y. R., Kim, Y., Streller, F., Carpick, R. W., Rappe, A. M., Drndić, M., Kikkawa, J. M., & Johnson, A. T. C.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-06-20
- Volume
- 16
- Issue
- 7
- Pages
- 4297-4304
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2404536606
- Cited by
- 222
- References
- 5
- FWCI
- 16.74
- Type
- journal article
- Language
- en
- Open access
- green
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- The paper
- Naylor, C. H., Parkin, W. M., Ping, J., Gao, Z., Zhou, Y. R., Kim, Y., Streller, F., Carpick, R. W., Rappe, A. M., Drndić, M., Kikkawa, J. M., & Johnson, A. T. C. (2016). Monolayer Single-Crystal 1T′-MoTe2 Grown by Chemical Vapor Deposition Exhibits Weak Antilocalization Effect. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b01342
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