The DOI matches its Crossref record; 37 of the 37 references it cites were found in a registry or an index.
Band Gap Engineering with Ultralarge Biaxial Strains in Suspended Monolayer MoS2
Open accessAbstract
We demonstrate the continuous and reversible tuning of the optical band gap of suspended monolayer MoS2 membranes by as much as 500 meV by applying very large biaxial strains. By using chemical vapor deposition (CVD) to grow crystals that are highly impermeable to gas, we are able to apply a pressure difference across suspended membranes to induce biaxial strains. We observe the effect of strain on the energy and intensity of the peaks in the photoluminescence (PL) spectrum and find a linear tuning rate of the optical band gap of 99 meV/%. This method is then used to study the PL spectra of bilayer and trilayer devices under strain and to find the shift rates and Grüneisen parameters of two Raman modes in monolayer MoS2. Finally, we use this result to show that we can apply biaxial strains as large as 5.6% across micron-sized areas and report evidence for the strain tuning of higher level optical transitions.
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Cites
Atomically Thin MoS 2 : A New Direct-Gap Semiconductor
Mak, K. F., Lee, C., Hone, J., Shan, J., & Heinz, T. F. (2010) · Physical Review Letters · doi:10.1103/physrevlett.105.136805 · Cited by 15,586
Radisavljevic, B., Radenovic, A., Brivio, J., Giacometti, V., & Kis, A. (2011) · Nature Nanotechnology · doi:10.1038/nnano.2010.279 · Cited by 14,939
Impermeable Atomic Membranes from Graphene Sheets
Bunch, J. S., Verbridge, S. S., Alden, J. S., van der Zande, A. M., Parpia, J. M., Craighead, H. G., & McEuen, P. L. (2008) · Nano Letters · doi:10.1021/nl801457b · Cited by 2,919
Self-citationTightly bound trions in monolayer MoS2
Mak, K. F., He, K., Lee, C., Lee, G. H., Hone, J., Heinz, T. F., & Shan, J. (2013) · Nature Materials · doi:10.1038/nmat3505 · Cited by 2,865
Stretching and Breaking of Ultrathin MoS2
Bertolazzi, S., Brivio, J., & Kis, A. (2011) · ACS Nano · doi:10.1021/nn203879f · Cited by 2,680
Bandgap Engineering of Strained Monolayer and Bilayer MoS2
Conley, H. J., Wang, B., Ziegler, J. I., Haglund, R. F., Pantelides, S. T., & Bolotin, K. I. (2013) · Nano Letters · doi:10.1021/nl4014748 · Cited by 2,497
Piezoelectricity of single-atomic-layer MoS2 for energy conversion and piezotronics
Wu, W., Wang, L., Li, Y., Zhang, F., Lin, L., Niu, S., Chenet, D., Zhang, X., Hao, Y., Heinz, T. F., et al. (2014) · Nature · doi:10.1038/nature13792 · Cited by 2,287
Transfer of CVD-Grown Monolayer Graphene onto Arbitrary Substrates
Suk, J. W., Kitt, A., Magnuson, C. W., Hao, Y., Ahmed, S., An, J., Swan, A. K., Goldberg, B. B., & Ruoff, R. S. (2011) · ACS Nano · doi:10.1021/nn201207c · Cited by 1,495
Self-citationMoS2 Nanosheet Phototransistors with Thickness-Modulated Optical Energy Gap
Lee, H. S., Min, S.-W., Chang, Y.-G., Park, M. K., Nam, T., Kim, H., Kim, J. H., Ryu, S., & Im, S. (2012) · Nano Letters · doi:10.1021/nl301485q · Cited by 1,337
Local Strain Engineering in Atomically Thin MoS2
Castellanos-Gomez, A., Roldán, R., Cappelluti, E., Buscema, M., Guinea, F., van der Zant, H. S. J., & Steele, G. A. (2013) · Nano Letters · doi:10.1021/nl402875m · Cited by 1,309
Cited by
Enhancing Electrocatalytic Water Splitting by Strain Engineering
You, B., Tang, M. T., Tsai, C., Abild‐Pedersen, F., Zheng, X., & Li, H. (2019) · Advanced Materials · doi:10.1002/adma.201807001 · Cited by 793
Metadata
- Authors
- Lloyd, D., Liu, X., Christopher, J. W., Cantley, L., Wadehra, A., Kim, B. L., Goldberg, B. B., Swan, A. K., & Bunch, J. S.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-08-15
- Volume
- 16
- Issue
- 9
- Pages
- 5836-5841
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2513056946
- Cited by
- 624
- References
- 37
- FWCI
- 19.79
- Type
- journal article
- Language
- en
- Open access
- green
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- Lloyd, D., Liu, X., Christopher, J. W., Cantley, L., Wadehra, A., Kim, B. L., Goldberg, B. B., Swan, A. K., & Bunch, J. S. (2016). Band Gap Engineering with Ultralarge Biaxial Strains in Suspended Monolayer MoS2. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b02615
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