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Ising-Type Magnetic Ordering in Atomically Thin FePS3
Open accessAbstract
Magnetism in two-dimensional materials is not only of fundamental scientific interest but also a promising candidate for numerous applications. However, studies so far, especially the experimental ones, have been mostly limited to the magnetism arising from defects, vacancies, edges, or chemical dopants which are all extrinsic effects. Here, we report on the observation of intrinsic antiferromagnetic ordering in the two-dimensional limit. By monitoring the Raman peaks that arise from zone folding due to antiferromagnetic ordering at the transition temperature, we demonstrate that FePS 3 exhibits an Ising-type antiferromagnetic ordering down to the monolayer limit, in good agreement with the Onsager solution for two-dimensional order–disorder transition. The transition temperature remains almost independent of the thickness from bulk to the monolayer limit with T N ∼ 118 K, indicating that the weak interlayer interaction has little effect on the antiferromagnetic ordering.
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Cites
Zur Theorie der Metalle: I. Eigenwerte und Eigenfunktionen der linearen Atomkette
Bethe, H. (1931) · Zeitschrift f�r Physik · doi:10.1007/bf01341708 · Cited by 3,768
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Multifunctional antiferromagnetic materials with giant piezomagnetism and noncollinear spin current
Ma, H.-Y., Hu, M., Li, N., Liu, J., Yao, W., Jia, J.-F., & Liu, J. (2021) · Nature Communications · doi:10.1038/s41467-021-23127-7 · Cited by 490
Suppression of magnetic ordering in XXZ-type antiferromagnetic monolayer NiPS3
Kim, K., Lim, S. Y., Lee, J.-U., Lee, S., Kim, T. Y., Park, K., Jeon, G. S., Park, C.-H., Park, J.-G., & Cheong, H. (2019) · Nature Communications · doi:10.1038/s41467-018-08284-6 · Cited by 452
Self-citationRecent progress on 2D magnets: Fundamental mechanism, structural design and modification
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Hard magnetic properties in nanoflake van der Waals Fe3GeTe2
Tan, C., Lee, J., Jung, S.-G., Park, T., Albarakati, S., Partridge, J., Field, M. R., McCulloch, D. G., Wang, L., & Lee, C. (2018) · Nature Communications · doi:10.1038/s41467-018-04018-w · Cited by 426
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Metadata
- Authors
- Lee, J.-U., Lee, S., Ryoo, J. H., Kang, S., Kim, T. Y., Kim, P., Park, C.-H., Park, J.-G., & Cheong, H.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-11-14
- Volume
- 16
- Issue
- 12
- Pages
- 7433-7438
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2509776654
- Cited by
- 1,074
- References
- 1
- FWCI
- 19.50
- Type
- journal article
- Language
- en
- Open access
- green
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- Lee, J.-U., Lee, S., Ryoo, J. H., Kang, S., Kim, T. Y., Kim, P., Park, C.-H., Park, J.-G., & Cheong, H. (2016). Ising-Type Magnetic Ordering in Atomically Thin FePS3. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b03052
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