The DOI matches its Crossref record; 2 of the 2 references it cites were found in a registry or an index.
Conformal, Nanoscale ZnO Surface Modification of Garnet-Based Solid-State Electrolyte for Lithium Metal Anodes
Abstract
Solid-state electrolytes are known for nonflammability, dendrite blocking, and stability over large potential windows. Garnet-based solid-state electrolytes have attracted much attention for their high ionic conductivities and stability with lithium metal anodes. However, high-interface resistance with lithium anodes hinders their application to lithium metal batteries. Here, we demonstrate an ultrathin, conformal ZnO surface coating by atomic layer deposition for improved wettability of garnet solid-state electrolytes to molten lithium that significantly decreases the interface resistance to as low as ∼20 Ω·cm 2 . The ZnO coating demonstrates a high reactivity with lithium metal, which is systematically characterized. As a proof-of-concept, we successfully infiltrated lithium metal into porous garnet electrolyte, which can potentially serve as a self-supported lithium metal composite anode having both high ionic and electrical conductivity for solid-state lithium metal batteries. The facile surface treatment method offers a simple strategy to solve the interface problem in solid-state lithium metal batteries with garnet solid electrolytes.
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Cites
Armand, M., & Tarascon, J.-M. (2008) · Nature · doi:10.1038/451652a · Cited by 19,612
Interface Stability in Solid-State Batteries
Richards, W. D., Miara, L. J., Wang, Y., Kim, J. C., & Ceder, G. (2016) · Chemistry of Materials · doi:10.1021/acs.chemmater.5b04082 · Cited by 1,652
Cited by
Designing solid-state electrolytes for safe, energy-dense batteries
Zhao, Q., Stalin, S., Zhao, C.-Z., & Archer, L. A. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0165-5 · Cited by 2,372
Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes
Banerjee, A., Wang, X., Fang, C., Wu, E. A., & Meng, Y. S. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00101 · Cited by 1,526
Gao, Z., Sun, H., Fu, L., Ye, F., Zhang, Y., Luo, W., & Huang, Y. (2018) · Advanced Materials · doi:10.1002/adma.201705702 · Cited by 1,300
Self-citationPhysicochemical Concepts of the Lithium Metal Anode in Solid-State Batteries
Krauskopf, T., Richter, F. H., Zeier, W. G., & Janek, J. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.0c00431 · Cited by 892
Recent Advances in Energy Chemistry between Solid-State Electrolyte and Safe Lithium-Metal Anodes
Cheng, X.-B., Zhao, C.-Z., Yao, Y.-X., Liu, H., & Zhang, Q. (2019) · Chem · doi:10.1016/j.chempr.2018.12.002 · Cited by 874
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Metadata
- Authors
- Wang, C., Gong, Y., Liu, B., Fu, K., Yao, Y., Hitz, E., Li, Y., Dai, J., Xu, S., Luo, W., Wachsman, E. D., & Hu, L.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-12-16
- Volume
- 17
- Issue
- 1
- Pages
- 565-571
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2562307633
- Cited by
- 682
- References
- 2
- FWCI
- 31.41
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, C., Gong, Y., Liu, B., Fu, K., Yao, Y., Hitz, E., Li, Y., Dai, J., Xu, S., Luo, W., Wachsman, E. D., & Hu, L. (2017). Conformal, Nanoscale ZnO Surface Modification of Garnet-Based Solid-State Electrolyte for Lithium Metal Anodes. Nano Letters. https://doi.org/10.1021/acs.nanolett.6b04695
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