The DOI matches its Crossref record; 3 of the 3 references it cites were found in a registry or an index.
Aqueous Zinc-Ion Storage in MoS2 by Tuning the Intercalation Energy
Abstract
Abstract Aqueous Zn-ion batteries present low-cost, safe, and high-energy battery technology but suffer from the lack of suitable cathode materials because of the sluggish intercalation kinetics associated with the large size of hydrated zinc ions. Herein we report an effective and general strategy to transform inactive intercalation hosts into efficient Zn2+ storage materials through intercalation energy tuning. Using MoS2 as a model system, we show both experimentally and theoretically that even hosts with an originally poor Zn2+ diffusivity can allow fast Zn2+ diffusion. Through simple interlayer spacing and hydrophilicity engineering that can be experimentally achieved by oxygen incorporation, the Zn2+ diffusivity is boosted by 3 orders of magnitude, effectively enabling the otherwise barely active MoS2 to achieve a high capacity of 232 mAh g–1, which is 10 times that of its pristine form. The strategy developed in our work can be generally applied for enhancing the ion storage capacity of metal chalcogenides and other layered materials, making them promising cathodes for challenging multivalent ion batteries.
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Cites
Electronics and optoelectronics of two-dimensional transition metal dichalcogenides
Wang, Q. H., Kalantar-Zadeh, K., Kis, A., Coleman, J. N., & Strano, M. S. (2012) · Nature Nanotechnology · doi:10.1038/nnano.2012.193 · Cited by 16,374
A review on the key issues for lithium-ion battery management in electric vehicles
Lu, L., Han, X., Li, J., Hua, J., & Ouyang, M. (2013) · Journal of Power Sources · doi:10.1016/j.jpowsour.2012.10.060 · Cited by 4,837
Xie, J., Zhang, J., Li, S., Grote, F., Zhang, X., Zhang, H., Wang, R., Lei, Y., Pan, B., & Xie, Y. (2013) · Journal of the American Chemical Society · doi:10.1021/ja408329q · Cited by 2,350
Cited by
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Liu, S., Zhu, H., Zhang, B., Li, G., Zhu, H., Ren, Y., Geng, H., Yang, Y., Liu, Q., & Li, C. C. (2020) · Advanced Materials · doi:10.1002/adma.202001113 · Cited by 561
Li, M., Li, Z., Wang, X., Meng, J., Liu, X., Wu, B., Han, C., & Mai, L. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00030f · Cited by 559
Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries
Wang, X., Zhang, Z., Xi, B., Chen, W., Jia, Y., Feng, J., & Xiong, S. (2021) · ACS Nano · doi:10.1021/acsnano.1c01389 · Cited by 531
He, H., Tong, H., Song, X., Song, X., & Liu, J. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta00748j · Cited by 512
Metadata
- Authors
- Liang, H., Cao, Z., Ming, F., Zhang, W., Anjum, D. H., Cui, Y., Cavallo, L., & Alshareef, H. N.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-04-15
- Volume
- 19
- Issue
- 5
- Pages
- 3199-3206
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2936088874
- Cited by
- 525
- References
- 3
- FWCI
- 24.67
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liang, H., Cao, Z., Ming, F., Zhang, W., Anjum, D. H., Cui, Y., Cavallo, L., & Alshareef, H. N. (2019). Aqueous Zinc-Ion Storage in MoS2 by Tuning the Intercalation Energy. Nano Letters. https://doi.org/10.1021/acs.nanolett.9b00697
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