The DOI matches its Crossref record; 4 of the 4 references it cites were found in a registry or an index.
Interface Modulation of Two-Dimensional Superlattices for Efficient Overall Water Splitting
Abstract
Molecular-scale modulation of interfaces between different unilamellar nanosheets in superlattices is promising for efficient catalytic activities. Here, three kinds of superlattices from alternate restacking of any two of the three unilamellar nanosheets of MoS 2, NiFe-layered double hydroxide (NiFe-LDH), and graphene are systematically investigated for electrocatalytic water splitting. The MoS 2 /NiFe-LDH superlattice exhibits a low overpotential of 210 and 110 mV at 10 mA cm –2 for oxygen evolution reaction (OER) and alkaline hydrogen evolution reaction (HER), respectively, superior than MoS 2 /graphene and NiFe-LDH/graphene superlattices. High activity and stability toward the overall water splitting are also demonstrated on the MoS 2 /NiFe-LDH superlattice bifunctional electrocatalyst, outperforming the commercial Pt/C-RuO 2 couple. This outstanding performance can be attributed to optimal adsorption energies of both HER and OER intermediates on the MoS 2 /NiFe-LDH superlattice, which originates from a strong electronic coupling effect at the heterointerfaces. These results herald the interface modulation of superlattices providing a promising approach for designing advanced electrocatalysts.
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Cites
Enhancing Hydrogen Evolution Activity in Water Splitting by Tailoring Li + -Ni(OH) 2 -Pt Interfaces
Subbaraman, R., Tripkovic, D., Strmcnik, D., Chang, K.-C., Uchimura, M., Paulikas, A. P., Stamenkovic, V., & Markovic, N. M. (2011) · Science · doi:10.1126/science.1211934 · Cited by 3,135
Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
Luo, J., Im, J.-H., Mayer, M. T., Schreier, M., Nazeeruddin, M. K., Park, N.-G., Tilley, S. D., Fan, H. J., & Grätzel, M. (2014) · Science · doi:10.1126/science.1258307 · Cited by 2,509
Ma, W., Ma, R., Wang, C., Liang, J., Liu, X., Zhou, K., & Sasaki, T. (2015) · ACS Nano · doi:10.1021/nn5069836 · Cited by 714
Self-citationZhu, Z., Yin, H., He, C., Al‐Mamun, M., Liu, P., Jiang, L., Zhao, Y., Wang, Y., Yang, H., Tang, Z., et al. (2018) · Advanced Materials · doi:10.1002/adma.201801171 · Cited by 228
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Cited by
Chatenet, M., Pollet, B. G., Dekel, D. R., Dionigi, F., Deseure, J., Millet, P., Braatz, R. D., Bazant, M. Z., Eikerling, M., Staffell, I., et al. (2022) · Chemical Society Reviews · doi:10.1039/d0cs01079k · Cited by 2,025
2D Transition Metal Dichalcogenides: Design, Modulation, and Challenges in Electrocatalysis
Fu, Q., Han, J., Wang, X., Xu, P., Yao, T., Zhong, J., Zhong, W., Liu, S., Gao, T., Zhang, Z., et al. (2021) · Advanced Materials · doi:10.1002/adma.201907818 · Cited by 697
Xu, Q., Zhang, J., Zhang, H., Zhang, L., Chen, L., Hu, Y., Jiang, H., & Li, C. (2021) · Energy & Environmental Science · doi:10.1039/d1ee02105b · Cited by 469
Self-citationCarbon quantum dots for advanced electrocatalysis
Tian, L., Li, Z., Wang, P., Zhai, X., Wang, X., & Li, T. (2021) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2020.06.057 · Cited by 384
Chen, J., Long, Q., Xiao, K., Ouyang, T., Li, N., Ye, S., & Liu, Z.-Q. (2021) · Science Bulletin · doi:10.1016/j.scib.2021.02.033 · Cited by 363
Metadata
- Authors
- Xiong, P., Zhang, X., Wan, H., Wang, S., Zhao, Y., Zhang, J., Zhou, D., Gao, W., Ma, R., Sasaki, T., & Wang, G.
- Venue
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Published
- 2019-06-03
- Volume
- 19
- Issue
- 7
- Pages
- 4518-4526
- ISSN
- 1530-6984 (ISSN-L)
- 1530-6992
- OpenAlex
- W2948325434
- Cited by
- 259
- References
- 4
- FWCI
- 7.83
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xiong, P., Zhang, X., Wan, H., Wang, S., Zhao, Y., Zhang, J., Zhou, D., Gao, W., Ma, R., Sasaki, T., & Wang, G. (2019). Interface Modulation of Two-Dimensional Superlattices for Efficient Overall Water Splitting. Nano Letters. https://doi.org/10.1021/acs.nanolett.9b01329
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