Cited by 191Advanced Photocatalysis TechniquesElectrocatalysts for Energy ConversionIron oxide chemistry and applications

Advanced Catalysts for Photoelectrochemical Water Splitting

Marwat, Mohsin Ali, Humayun, Muhammad, Afridi, Muhammad Waqas, Zhang, Haibo, Abdul Karim, Muhammad Ramzan, Ashtar, Malik, Usman, Muhammad, Waqar, Saad +3 more·2021·ACS Applied Energy Materials

Abstract

Photoelectrochemical (PEC) water splitting offers a sparkling and sustainable strategy for hydrogen generation, and significant research for enhancing the conversion efficiency of electrocatalysts is underway, since a huge number of publications have been reported in this field. Hence, it is urgent to write a comprehensive and updated review in order to highlight the latest progress in the design, fabrication, and modification of electrocatalysts for high-efficiency PEC water splitting. In this review, we describe the basic mechanism of PEC water splitting utilizing electrocatalysts in detail. Further, we highlighted the recent advancements in the design, fabrication, and modification of high-efficiency electrocatalysts for energy conversion. In addition, the catalysts’ surface passivation, heterojunction constructions, defect engineering, and photovoltage and photocurrent enhancements are also highlighted.

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Registry

Crossref · 10.1021/acsaem.1c02548

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  • The low electronic conductivity, wide band gap, rapid charge carrier recombination, and small accessible surface active sites of carbon nitride greatly limit its application in water splitting and photosynthesis.

    “Unfortunately, the low electronic conductivity, wide band gap, rapid charge carrier recombination behavior, as well as the fairly small accessible surface active sites, have greatly limited its application in water splitting and photosynthesis [6, 7].”

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Authors
Marwat, M. A., Humayun, M., Afridi, M. W., Zhang, H., Abdul Karim, M. R., Ashtar, M., Usman, M., Waqar, S., Ullah, H., Wang, C., & Luo, W.
Affiliations
  • Ghulam Ishaq Khan Institute of Engineering Sciences and Technology (PK)
  • Wuhan National Laboratory for Optoelectronics (CN)
  • State Key Laboratory of Materials Processing and Die & Mould Technology (CN)
  • Department of Materials Science and Engineering, Ghulam Ishaq Khan Institute of Engineering Sciences and Technology, Topi 23640, Khyber Pakhtunkhwa, Pakistan
  • Huazhong University of Science and Technology (CN)
  • King Fahd University of Petroleum and Minerals (SA)
  • Shandong University (CN)
  • Wuhan University of Technology (CN)
Corresponding author
  • Wang, Chundong
  • Luo, Wei
Venue
ACS Applied Energy Materials
Published
2021-10-26
Volume
4
Issue
11
Pages
12007-12031
ISSN
2574-0962 (ISSN-L)
OpenAlex
W3209712157
Cited by
191
References
0
Citations by year
2026: 17 · 2025: 44 · 2024: 45 · 2023: 56 · 2022: 29
FWCI
6.10
Type
journal article
Language
en
Open access
closed
Locations
ACS Applied Energy Materials (publishedVersion)
Funders
  • Ministry of Science and Technology of the People's Republic of China (2017YFE0120500, 2018YFA0702100)
  • Saudi Aramco (ORCP2390)
  • National Natural Science Foundation of China (11874169, 51972129)
  • South Xinjiang Innovation and Development Program of Key Industries of Xinjiang Production and Construction Corps (2020DB002)
  • Hubei Province (2020BAB079)
Topics
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Iron oxide chemistry and applications
Keywords
photoelectrochemical water splitting, electrocatalysts, hydrogen production, surface passivation, heterojunction, defect engineering, photovoltage enhancement, photocurrent enhancement, energy conversion

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