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Facile Photochemical Synthesis of Au/Pt/g-C3N4with Plasmon-Enhanced Photocatalytic Activity for Antibiotic Degradation
Abstract
A novel plasmonic photocatalyst, Au/Pt/g-C3N4, was prepared by a facile calcination-photodeposition technique. The samples were characterized by X-ray diffraction, energy-dispersive spectroscopy, transmission electron microscopy, and UV-vis diffuse reflectance spectroscopy, and the results demonstrated that the Au and Pt nanoparticles (7-15 nm) were well-dispersed on the surfaces of g-C3N4. The Au/Pt codecorated g-C3N4 heterostructure displayed enhanced photocatalytic activity for antibiotic tetracycline hydrochloride (TC-HCl) degradation, and the degradation rate was 3.4 times higher than that of pure g-C3N4 under visible light irradiation. The enhancement of photocatalytic activity could be attributed to the surface plasmon resonance effect of Au and electron-sink function of Pt nanoparticles, which improve the optical absorption property and photogenerated charge carriers separation of g-C3N4, synergistically facilitating the photocatalysis process. Finally, a possible photocatalytic mechanism for degrading TC-HCl by Au/Pt/g-C3N4 heterostructure was tentatively proposed.
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Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
Enhanced disinfection application of Ag-modified g-C3N4 composite under visible light
Ma, S., Zhan, S., Jia, Y., Shi, Q., & Zhou, Q. (2016) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2015.12.051 · Cited by 420
Self-citationMolecularly imprinted polymers by the surface imprinting technique
Dong, C., Shi, H., Han, Y., Yang, Y., Wang, R., & Men, J. (2021) · European Polymer Journal · doi:10.1016/j.eurpolymj.2020.110231 · Cited by 365
Zhang, S., Liu, Y., Gu, P., Ma, R., Wen, T., Zhao, G., Li, L., Ai, Y., Hu, C., & Wang, X. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.02.008 · Cited by 361
Li, X., Cui, K., Guo, Z., Yang, T., Cao, Y., Xiang, Y., Chen, H., & Xi, M. (2020) · Chemical Engineering Journal · doi:10.1016/j.cej.2019.122324 · Cited by 308
Metadata
- Authors
- Xue, J., Ma, S., Zhou, Y., Zhang, Z., & He, M.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-04-28
- Volume
- 7
- Issue
- 18
- Pages
- 9630-9637
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2329540166
- Cited by
- 667
- References
- 0
- FWCI
- 17.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Xue, J., Ma, S., Zhou, Y., Zhang, Z., & He, M. (2015). Facile Photochemical Synthesis of Au/Pt/g-C3N4with Plasmon-Enhanced Photocatalytic Activity for Antibiotic Degradation. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b01212
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