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Self-Assembly Synthesis of N-Doped Carbon Aerogels for Supercapacitor and Electrocatalytic Oxygen Reduction
Abstract
The rational design of high-performance and cheap nanomaterials for multiple sustainable energy storage applications is extremely urgent but remains challenging. Herein, a facile commercial melamine-sponge-directed multicomponent surface self-assembly strategy has been reported to synthesize N-doped carbon aerogels (NCAs) with low density (0.01 g cm(-3)), large open pores, and high surface area (1626 m2 g(-1)). The commercial melamine sponge simultaneously serves as a green N source for N-doping and a 3D scaffold to buffer electrolytes for reducing ion transport resistance and minimizing ion diffusion distance. With their tailored architecture characteristics, the NCAs-based supercapacitor and oxygen reduction electrocatalyst show excellent performance.
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CAs exhibit anaerobic stability and little interfacial contact resistance, and have perfect electrical conductivity and biocompatible porosity derived from the tunable 3D hierarchical morphology with ultrafine sizes and conductive framework.
“Thus, CAs exhibit not only have anaerobic stability and little interfacial contact resistance, but also the perfect electrical conductivity and biocompatible porosity derived from the tunable 3D hierarchical morphology with ultrafine sizes and conductive framework [31,33].”
From Self-supported microbial carbon aerogel bioelectrocatalytic anode promoting extracellular electron transfer for efficient hydrogen evolution (2019) · cites this paper as [33]
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Sorted by citations
Nitrogen-doped porous carbon/graphene aerogel with much enhanced capacitive behaviors
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Metadata
- Authors
- Zhang, J., Chen, G., Zhang, Q., Kang, F., & You, B.
- Affiliations
- University of Science and Technology of China (CN)
- Utah State University (US)
- Corresponding author
- You, Bo
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-06-05
- Volume
- 7
- Issue
- 23
- Pages
- 12760-12766
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W789695241
- Cited by
- 119
- References
- 1
- Citations by year
- 2026: 5 · 2025: 6 · 2024: 8 · 2023: 5 · 2022: 6 · 2021: 9 · 2020: 4 · 2019: 16 · 2018: 18 · 2017: 19 · 2016: 16 · 2015: 7
- FWCI
- 6.54
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ACS Applied Materials & Interfaces (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Aerogels and thermal insulation
- Keywords
- self-assembly synthesis, melamine sponge, supercapacitors, oxygen reduction reaction, electrocatalysts, nitrogen doping, porous carbon, ion transport resistance, energy storage
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