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Hydrothermal Synthesis g-C3N4/Nano-InVO4 Nanocomposites and Enhanced Photocatalytic Activity for Hydrogen Production under Visible Light Irradiation
Abstract
We synthesized g-C3N4/nano-InVO4 heterojunction-type photocatalyts by in situ growth of InVO4 nanoparticles onto the surface of g-C3N4 sheets via a hydrothermal process. The results of SEM and TEM showed that the obtained InVO4 nanoparticles 20 nm in size dispersed uniformly on the surface of g-C3N4 sheets, which revealed that g-C3N4 sheets was probably a promising support for in situ growth of nanosize materials. The achieved intimate interface promoted the charge transfer and inhibited the recombination rate of photogenerated electron-hole pairs, which significantly improved the photocatalytic activity. A possible growth process of g-C3N4/nano-InVO4 nanocomposites was proposed based on different mass fraction of g-C3N4 content. The obtained g-C3N4/nano-InVO4 nanocomposites could achieve effective separation of charge-hole pairs and stronger reducing power, which caused enhanced H2 evolution from water-splitting compared with bare g-C3N4 sheets and g-C3N4/micro-InVO4 composites, respectively. As a result, the g-C3N4/nano-InVO4 nanocomposite with a mass ratio of 80:20 possessed the maximum photocatalytic activity for hydrogen production under visible-light irradiation.
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Citations
Cites
Semiconductor-based Photocatalytic Hydrogen Generation
Chen, X., Shen, S., Guo, L., & Mao, S. S. (2010) · Chemical Reviews · doi:10.1021/cr1001645 · Cited by 7,876
Abe, R. (2010) · Journal of Photochemistry and Photobiology C: Photochemistry Reviews · doi:10.1016/j.jphotochemrev.2011.02.003 · Cited by 1,223
Iwashina, K., & Kudo, A. (2011) · Journal of the American Chemical Society · doi:10.1021/ja2050315 · Cited by 457
Cited by
Ong, W.-J., Tan, L.-L., Ng, Y. H., Yong, S.-T., & Chai, S.-P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00075 · Cited by 7,147
g‐C3N4‐Based Heterostructured Photocatalysts
Fu, J., Yu, J., Jiang, C., & Cheng, B. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201701503 · Cited by 2,565
Liao, G., Gong, Y., Zhang, L., Gao, H., Yang, G.-J., & Fang, B. (2019) · Energy & Environmental Science · doi:10.1039/c9ee00717b · Cited by 1,075
Ye, R., Fang, H., Zheng, Y.-Z., Li, N., Wang, Y., & Tao, X. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b01850 · Cited by 420
Recent development in graphitic carbon nitride based photocatalysis for hydrogen generation
Nasir, M. S., Yang, G., Ayub, I., Wang, S., Wang, L., Wang, X., Yan, W., Peng, S., & Ramakarishna, S. (2019) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2019.117855 · Cited by 351
Metadata
- Authors
- Hu, B., Cai, F., Chen, T., Fan, M., Song, C., Yan, X., & Shi, W.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-08-17
- Volume
- 7
- Issue
- 33
- Pages
- 18247-18256
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2338638442
- Cited by
- 206
- References
- 3
- FWCI
- 6.84
- Type
- journal article
- Language
- en
- Open access
- closed
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- Hu, B., Cai, F., Chen, T., Fan, M., Song, C., Yan, X., & Shi, W. (2015). Hydrothermal Synthesis g-C3N4/Nano-InVO4 Nanocomposites and Enhanced Photocatalytic Activity for Hydrogen Production under Visible Light Irradiation. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b05715
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