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Mixed-Metal–Organic Framework with Effective Lewis Acidic Sites for Sulfur Confinement in High-Performance Lithium–Sulfur Batteries
Abstract
The mixed-metal-organic framework approach and a representative zirconium-metalloporphyrin framework (MOF-525) have been developed to create novel sulfur hosts and Li-S batteries. The different local environments at the centers of the porphyrin moieties in a series of MMOFs-MOF-525(2H), MOF-525(FeCl), and MOF-525(Cu)-have led to their different behaviors for the confinement of sulfur and thus Li-S batteries. The unique structure of MOF-525(Cu) has enabled each Cu(2+) site to offer two Lewis acidic sites, featuring it as a very powerful MOF host for the inclusion of sulfur and polysulfides. The S@MOF-525(Cu) cathode has demonstrated the best performance among all reported sulfur/MOFs composite cathode materials, with a reversible capacity of about 700 mAh/g at 0.5 C after 200 cycles.
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Cites
Metal–organic frameworks as platforms for clean energy
Li, S.-L., & Xu, Q. (2013) · Energy & Environmental Science · doi:10.1039/c3ee40507a · Cited by 970
Cited by
Pristine Metal–Organic Frameworks and their Composites for Energy Storage and Conversion
Liang, Z., Qu, C., Guo, W., Zou, R., & Xu, Q. (2018) · Advanced Materials · doi:10.1002/adma.201702891 · Cited by 787
A novel synergistic composite with multi-functional effects for high-performance Li–S batteries
Li, Y.-J., Fan, J.-M., Zheng, M.-S., & Dong, Q.-F. (2016) · Energy & Environmental Science · doi:10.1039/c6ee00104a · Cited by 600
Mao, Y., Li, G., Guo, Y., Li, Z., Liang, C., Peng, X., & Lin, Z. (2017) · Nature Communications · doi:10.1038/ncomms14628 · Cited by 518
Metal–Organic Frameworks (MOFs) and MOF-Derived Materials for Energy Storage and Conversion
Zhang, X., Chen, A., Zhong, M., Zhang, Z., Zhang, X., Zhou, Z., & Bu, X.-H. (2019) · Electrochemical Energy Reviews · doi:10.1007/s41918-018-0024-x · Cited by 481
Metal–organic framework composites and their electrochemical applications
Xue, Y., Zheng, S., Xue, H., & Pang, H. (2019) · Journal of Materials Chemistry A · doi:10.1039/c8ta12178h · Cited by 389
Metadata
- Authors
- Wang, Z., Wang, B., Yang, Y., Cui, Y., Wang, Z., Chen, B., & Qian, G.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-09-08
- Volume
- 7
- Issue
- 37
- Pages
- 20999-21004
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W1255788758
- Cited by
- 218
- References
- 1
- FWCI
- 8.34
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, Z., Wang, B., Yang, Y., Cui, Y., Wang, Z., Chen, B., & Qian, G. (2015). Mixed-Metal–Organic Framework with Effective Lewis Acidic Sites for Sulfur Confinement in High-Performance Lithium–Sulfur Batteries. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b07024
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