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Origin of Electrochemical, Structural, and Transport Properties in Nonaqueous Zinc Electrolytes
Open accessAbstract
Through coupled experimental analysis and computational techniques, we uncover the origin of anodic stability for a range of nonaqueous zinc electrolytes. By examination of electrochemical, structural, and transport properties of nonaqueous zinc electrolytes with varying concentrations, it is demonstrated that the acetonitrile-Zn(TFSI)2, acetonitrile-Zn(CF3SO3)2, and propylene carbonate-Zn(TFSI)2 electrolytes can not only support highly reversible Zn deposition behavior on a Zn metal anode (≥99% of Coulombic efficiency) but also provide high anodic stability (up to ∼3.8 V vs Zn/Zn(2+)). The predicted anodic stability from DFT calculations is well in accordance with experimental results, and elucidates that the solvents play an important role in anodic stability of most electrolytes. Molecular dynamics (MD) simulations were used to understand the solvation structure (e.g., ion solvation and ionic association) and its effect on dynamics and transport properties (e.g., diffusion coefficient and ionic conductivity) of the electrolytes. The combination of these techniques provides unprecedented insight into the origin of the electrochemical, structural, and transport properties in nonaqueous zinc electrolytes.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
High rate and stable cycling of lithium metal anode
Qian, J., Henderson, W. A., Xu, W., Bhattacharya, P., Engelhard, M., Borodin, O., & Zhang, J.-G. (2015) · Nature Communications · doi:10.1038/ncomms7362 · Cited by 2,561
Cited by
Highly reversible zinc metal anode for aqueous batteries
Wang, F., Borodin, O., Gao, T., Fan, X., Sun, W., Han, F., Faraone, A., Dura, J. A., Xu, K., & Wang, C. (2018) · Nature Materials · doi:10.1038/s41563-018-0063-z · Cited by 3,305
Scientific Challenges for the Implementation of Zn-Ion Batteries
Blanc, L. E., Kundu, D., & Nazar, L. F. (2020) · Joule · doi:10.1016/j.joule.2020.03.002 · Cited by 2,113
Zhang, N., Cheng, F., Liu, Y., Zhao, Q., Lei, K., Chen, C., Liu, X., & Chen, J. (2016) · Journal of the American Chemical Society · doi:10.1021/jacs.6b05958 · Cited by 1,886
Reversible epitaxial electrodeposition of metals in battery anodes
Zheng, J., Zhao, Q., Tang, T., Yin, J., Quilty, C. D., Renderos, G. D., Liu, X., Deng, Y., Wang, L., Bock, D. C., et al. (2019) · Science · doi:10.1126/science.aax6873 · Cited by 1,877
Current status and future directions of multivalent metal-ion batteries
Liang, Y., Dong, H., Aurbach, D., & Yao, Y. (2020) · Nature Energy · doi:10.1038/s41560-020-0655-0 · Cited by 1,521
Metadata
- Authors
- Han, S.-D., Rajput, N. N., Qu, X., Pan, B., He, M., Ferrandon, M. S., Liao, C., Persson, K. A., & Burrell, A. K.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-01-29
- Volume
- 8
- Issue
- 5
- Pages
- 3021-3031
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2262222115
- Cited by
- 242
- References
- 3
- FWCI
- 5.79
- Type
- journal article
- Language
- en
- Open access
- green
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- Han, S.-D., Rajput, N. N., Qu, X., Pan, B., He, M., Ferrandon, M. S., Liao, C., Persson, K. A., & Burrell, A. K. (2016). Origin of Electrochemical, Structural, and Transport Properties in Nonaqueous Zinc Electrolytes. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b10024
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