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Large-Scale, Highly Efficient, and Green Liquid-Exfoliation of Black Phosphorus in Ionic Liquids
Abstract
We developed a facile, large-scale, and environmentally friendly liquid-exfoliation method to produce stable and high-concentration dispersions of mono- to few-layer black phosphorus (BP) nanosheets from bulk BP using nine ionic liquids. The prepared suspensions can stabilize without any obvious sedimentation and aggregation in ambient air for one month. In particular, the concentration (up to 0.95 mg mL(-1)) of BP nanoflakes obtained in 1-hydroxyethyl-3-methylimidazolium trifluoromethansulfonate ([HOEMIM][TfO]) is the highest reported for BP nanosheets dispersions. This work provides new opportunities for preparing atomically thin BP nanosheets in green, large-scale, and highly concentrated processes and achieving its in situ application.
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The chemistry of two-dimensional layered transition metal dichalcogenide nanosheets
Chhowalla, M., Shin, H. S., Eda, G., Li, L.-J., Loh, K. P., & Zhang, H. (2013) · Nature Chemistry · doi:10.1038/nchem.1589 · Cited by 10,034
Cited by
Recent progress in 2D group-VA semiconductors: from theory to experiment
Zhang, S., Guo, S., Chen, Z., Wang, Y., Gao, H., Gómez-Herrero, J., Ares, P., Zamora, F., Zhu, Z., & Zeng, H. (2018) · Chemical Society Reviews · doi:10.1039/c7cs00125h · Cited by 850
Li, B., Lai, C., Zeng, G., Huang, D., Qin, L., Zhang, M., Cheng, M., Liu, X., Yi, H., Zhou, C., et al. (2019) · Small · doi:10.1002/smll.201804565 · Cited by 367
Emerging Trends in Phosphorene Fabrication towards Next Generation Devices
Dhanabalan, S. C., Ponraj, J. S., Guo, Z., Li, S., Bao, Q., & Zhang, H. (2017) · Advanced Science · doi:10.1002/advs.201600305 · Cited by 344
Scalable exfoliation and dispersion of two-dimensional materials – an update
Tao, H., Zhang, Y., Gao, Y., Sun, Z., Yan, C., & Texter, J. (2017) · Physical Chemistry Chemical Physics · doi:10.1039/c6cp06813h · Cited by 317
Li, Q., Zhou, Q., Shi, L., Chen, Q., & Wang, J. (2019) · Journal of Materials Chemistry A · doi:10.1039/c8ta10306b · Cited by 266
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Metadata
- Authors
- Zhao, W., Xue, Z., Wang, J., Jiang, J., Zhao, X., & Mu, T.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-12-09
- Volume
- 7
- Issue
- 50
- Pages
- 27608-27612
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2336081837
- Cited by
- 200
- References
- 1
- FWCI
- 7.73
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, W., Xue, Z., Wang, J., Jiang, J., Zhao, X., & Mu, T. (2015). Large-Scale, Highly Efficient, and Green Liquid-Exfoliation of Black Phosphorus in Ionic Liquids. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b10734
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