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Lanthanum Nitrate As Electrolyte Additive To Stabilize the Surface Morphology of Lithium Anode for Lithium–Sulfur Battery
Abstract
Lithium-sulfur (Li-S) battery is regarded as one of the most promising candidates beyond conventional lithium ion batteries. However, the instability of the metallic lithium anode during lithium electrochemical dissolution/deposition is still a major barrier for the practical application of Li-S battery. In this work, lanthanum nitrate, as electrolyte additive, is introduced into Li-S battery to stabilize the surface of lithium anode. By introducing lanthanum nitrate into electrolyte, a composite passivation film of lanthanum/lithium sulfides can be formed on metallic lithium anode, which is beneficial to decrease the reducibility of metallic lithium and slow down the electrochemical dissolution/deposition reaction on lithium anode for stabilizing the surface morphology of metallic Li anode in lithium-sulfur battery. Meanwhile, the cycle stability of the fabricated Li-S cell is improved by introducing lanthanum nitrate into electrolyte. Apparently, lanthanum nitrate is an effective additive for the protection of lithium anode and the cycling stability of Li-S battery.
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Citations
Cited by
Zhang, H., Eshetu, G. G., Judez, X., Li, C., Rodriguez‐Martínez, L. M., & Armand, M. (2018) · Angewandte Chemie International Edition · doi:10.1002/anie.201712702 · Cited by 774
Advanced Micro/Nanostructures for Lithium Metal Anodes
Zhang, R., Li, N., Cheng, X., Yin, Y., Zhang, Q., & Guo, Y. (2017) · Advanced Science · doi:10.1002/advs.201600445 · Cited by 549
Aqueous Batteries Operated at −50 °C
Nian, Q., Wang, J., Liu, S., Sun, T., Zheng, S., Zhang, Y., Tao, Z., & Chen, J. (2019) · Angewandte Chemie International Edition · doi:10.1002/anie.201908913 · Cited by 426
Self-citationA review of recent developments in rechargeable lithium–sulfur batteries
Kang, W., Deng, N., Ju, J., Li, Q., Wu, D., Ma, X., Li, L., Naebe, M., & Cheng, B. (2016) · Nanoscale · doi:10.1039/c6nr04923k · Cited by 391
How to avoid dendrite formation in metal batteries: Innovative strategies for dendrite suppression
Aslam, M. K., Niu, Y., Hussain, T., Tabassum, H., Tang, W., Xu, M., & Ahuja, R. (2021) · Nano Energy · doi:10.1016/j.nanoen.2021.106142 · Cited by 308
Metadata
- Authors
- Liu, S., Li, G.-R., & Gao, X.-P.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-21
- Volume
- 8
- Issue
- 12
- Pages
- 7783-7789
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2322290801
- Cited by
- 177
- References
- 0
- FWCI
- 10.21
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, S., Li, G.-R., & Gao, X.-P. (2016). Lanthanum Nitrate As Electrolyte Additive To Stabilize the Surface Morphology of Lithium Anode for Lithium–Sulfur Battery. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.5b12231
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