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High-Flux Positively Charged Nanocomposite Nanofiltration Membranes Filled with Poly(dopamine) Modified Multiwall Carbon Nanotubes
Abstract
The poor dispensability of pristine carbon nanotubes in water impedes their implications in thin-film nanocomposite membranes for crucial utilities such as water purification. In this work, high-flux positively charged nanocomposite nanofiltration membranes were exploited by uniformly embedding poly(dopamine) modified multiwall carbon nanotubes (PDA-MWCNTs) in polyamide thin-film composite membranes. With poly(dopamine) modification, fine dispersion of MWCNTs in polyethyleneimine (PEI) aqueous solutions was achieved, which was interracially polymerized with trimesoyl chloride (TMC) n-hexane solutions to prepare nanocomposite membranes. The compatibility and interactions between modified MWCNTs and polyamide matrix were enhanced, attributed to the poly(dopamine) coatings on MWCNT surfaces, leading to significantly improved water permeability. At optimized conditions, pure water permeability of the PEI/PDA-MWCNTs/TMC nanofiltration membrane (M-4) was 15.32 L m(-2) h(-1) bar(-1), which was ∼1.6 times increased compared with that of pristine PEI/TMC membranes. Salt rejection of M-4 to different multivalent cations decreased in the sequence ZnCl2 (93.0%) > MgCl2 (91.5%) > CuCl2 (90.5%) ≈ CaCl2, which is well-suited for water softening and heavy metal ion removal.
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Cites
Mussel-inspired surface chemistry for multifunctional coatings
Lee, H., Dellatore, S. M., Miller, W. M., & Messersmith, P. B. (2007) · Science · doi:10.1126/science.1147241 · Cited by 10,965
Phenomenological Theory of Ion Solvation. Effective Radii of Hydrated Ions
Nightingale, E. R. (1959) · The Journal of Physical Chemistry · doi:10.1021/j150579a011 · Cited by 3,505
Cross-Linking in Adhesive Quinoproteins: Studies with Model Decapeptides
Burzio, L. A., & Waite, J. H. (2000) · Biochemistry · doi:10.1021/bi0002434 · Cited by 485
Cited by
Zhang, Y., Wang, L., Sun, W., Hu, Y., & Tang, H. (2020) · Journal of Industrial and Engineering Chemistry · doi:10.1016/j.jiec.2019.09.002 · Cited by 344
How to coordinate the trade-off between water permeability and salt rejection in nanofiltration?
Zhang, R., Tian, J., Gao, S., & Van der Bruggen, B. (2020) · Journal of Materials Chemistry A · doi:10.1039/d0ta02510k · Cited by 268
Metadata
- Authors
- Zhao, F.-Y., Ji, Y.-L., Weng, X.-D., Mi, Y.-F., Ye, C.-C., An, Q.-F., & Gao, C.-J.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-03-01
- Volume
- 8
- Issue
- 10
- Pages
- 6693-6700
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2283987916
- Cited by
- 353
- References
- 3
- FWCI
- 25.26
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhao, F.-Y., Ji, Y.-L., Weng, X.-D., Mi, Y.-F., Ye, C.-C., An, Q.-F., & Gao, C.-J. (2016). High-Flux Positively Charged Nanocomposite Nanofiltration Membranes Filled with Poly(dopamine) Modified Multiwall Carbon Nanotubes. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.6b00394
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