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High-Yield Production of Boron Nitride Nanosheets and Its Uses as a Catalyst Support for Hydrogenation of Nitroaromatics
Abstract
Single- or few-layered h-BN nanosheets (BNNSs) are analogous to graphene and possess unique properties. However, their technological applications were severely hindered by the low production efficiency of BNNSs. We reported here a study in which BNNSs were efficiently produced by exfoliating bulk h-BN powder in thionyl chloride without using any dispersion agents. The BNNSs yield was as high as 20%, and it could be doubled through the second round of exfoliation of the h-BN precipitate. Microscopic results revealed that the BNNSs generally consisted of 3-20 layers. Pd nanoparticles were successfully immobilized and uniformly distributed on BNNS surfaces through the deposition-precipitation method. The resultant Pd-BNNS catalyst exhibited high catalytic activity and recyclability for the hydrogenation of nitro aromatics, demonstrating that BNNSs served as a promising platform to fabricate heterogeneous catalysts.
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Cites
Superior Thermal Conductivity of Single-Layer Graphene
Balandin, A. A., Ghosh, S., Bao, W., Calizo, I., Teweldebrhan, D., Miao, F., & Lau, C. N. (2008) · Nano Letters · doi:10.1021/nl0731872 · Cited by 13,823
Cited by
Zhao, J., & Chen, Z. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b05213 · Cited by 1,249
Structure, Properties and Applications of Two‐Dimensional Hexagonal Boron Nitride
Roy, S., Zhang, X., Puthirath, A. B., Meiyazhagan, A., Bhattacharyya, S., Rahman, M. M., Babu, G., Susarla, S., Saju, S. K., Tran, M. K., et al. (2021) · Advanced Materials · doi:10.1002/adma.202101589 · Cited by 871
Morishita, T., & Okamoto, H. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b08404 · Cited by 257
Soluble, Exfoliated Two-Dimensional Nanosheets as Excellent Aqueous Lubricants
Zhang, W., Cao, Y., Tian, P., Guo, F., Tian, Y., Zheng, W., Ji, X., & Liu, J. (2016) · ACS Applied Materials & Interfaces · doi:10.1021/acsami.6b09752 · Cited by 103
Metadata
- Authors
- Sun, W., Meng, Y., Fu, Q., Wang, F., Wang, G., Gao, W., Huang, X., & Lu, F.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-04-11
- Volume
- 8
- Issue
- 15
- Pages
- 9881-9888
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2313254188
- Cited by
- 210
- References
- 1
- FWCI
- 9.46
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sun, W., Meng, Y., Fu, Q., Wang, F., Wang, G., Gao, W., Huang, X., & Lu, F. (2016). High-Yield Production of Boron Nitride Nanosheets and Its Uses as a Catalyst Support for Hydrogenation of Nitroaromatics. ACS Applied Materials & Interfaces. https://doi.org/10.1021/acsami.6b01008
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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